Catalytic hydroxylation using chloroplatinum compounds
Using “PtCl 4” as the Pt(IV) component in the mixture of aqueous chloroPt(II)/chloroPt(IV) compounds makes the “Shilov” functionalization of alkyl groups considerably faster and more chemoselective to alcohols, and adding hydrogen peroxide re-oxidizes the Pt(II) reduction product to Pt(IV). Run in t...
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| Published in | Journal of molecular catalysis. A, Chemical Vol. 189; no. 1; pp. 17 - 22 |
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| Main Authors | , , |
| Format | Journal Article |
| Language | English |
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Elsevier B.V
16.10.2002
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| Abstract | Using “PtCl
4” as the Pt(IV) component in the mixture of aqueous chloroPt(II)/chloroPt(IV) compounds makes the “Shilov” functionalization of alkyl groups considerably faster and more chemoselective to alcohols, and adding hydrogen peroxide re-oxidizes the Pt(II) reduction product to Pt(IV). Run in this manner, the reaction system is long-lived and catalytic in platinum.
Using “PtCl
4” as the Pt(IV) component in the mixture of aqueous chloroPt(II)/chloroPt(IV) compounds makes the “Shilov” functionalization of alkyl groups considerably faster and more chemoselective to alcohols, and adding hydrogen peroxide re-oxidizes the Pt(II) reduction product to Pt(IV). Run in this manner, the reaction system is long-lived and catalytic in platinum. |
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| AbstractList | Using “PtCl
4” as the Pt(IV) component in the mixture of aqueous chloroPt(II)/chloroPt(IV) compounds makes the “Shilov” functionalization of alkyl groups considerably faster and more chemoselective to alcohols, and adding hydrogen peroxide re-oxidizes the Pt(II) reduction product to Pt(IV). Run in this manner, the reaction system is long-lived and catalytic in platinum.
Using “PtCl
4” as the Pt(IV) component in the mixture of aqueous chloroPt(II)/chloroPt(IV) compounds makes the “Shilov” functionalization of alkyl groups considerably faster and more chemoselective to alcohols, and adding hydrogen peroxide re-oxidizes the Pt(II) reduction product to Pt(IV). Run in this manner, the reaction system is long-lived and catalytic in platinum. |
| Author | Thorn, D.L. Roe, D.C. DeVries, N. |
| Author_xml | – sequence: 1 givenname: N. surname: DeVries fullname: DeVries, N. – sequence: 2 givenname: D.C. surname: Roe fullname: Roe, D.C. – sequence: 3 givenname: D.L. surname: Thorn fullname: Thorn, D.L. |
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| Cites_doi | 10.1016/0022-328X(95)05567-9 10.1021/om00027a045 10.3891/acta.chem.scand.29a-0499 10.1021/ja00082a022 10.1021/ja960110z 10.1002/(SICI)1521-3773(19980904)37:16<2180::AID-ANIE2180>3.0.CO;2-A 10.1021/cr9411886 10.1126/science.280.5363.560 10.1021/ja001926+ 10.1016/S1381-1169(96)00118-5 10.1021/ja00770a065 10.1039/c39930000970 10.1021/ja016280f 10.1021/ja971952g 10.1016/S0010-8545(00)80523-8 10.1021/ja9620595 10.1016/0304-5102(93)E0230-E 10.1021/ja984028a 10.1021/ba-1992-0230.ch015 10.1021/ic00062a029 10.1021/ja00042a014 10.1007/0-306-46945-6 10.1021/ic50090a030 10.1016/0022-328X(95)05568-A 10.1039/C39910001242 10.1016/0277-5387(94)00329-D |
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Soc. doi: 10.1021/ja00042a014 contributor: fullname: Sen – ident: 10.1016/S1381-1169(02)00194-2_BIB1 doi: 10.1007/0-306-46945-6 – ident: 10.1016/S1381-1169(02)00194-2_BIB4 – volume: 9 start-page: 1927 year: 1970 ident: 10.1016/S1381-1169(02)00194-2_BIB26 publication-title: Inorg. Chem. doi: 10.1021/ic50090a030 contributor: fullname: Cox – volume: 504 start-page: 69 year: 1995 ident: 10.1016/S1381-1169(02)00194-2_BIB6 publication-title: J. Organomet. Chem. doi: 10.1016/0022-328X(95)05568-A contributor: fullname: Hutson – ident: 10.1016/S1381-1169(02)00194-2_BIB10 doi: 10.1039/C39910001242 – volume: 14 start-page: 197 year: 1995 ident: 10.1016/S1381-1169(02)00194-2_BIB12 publication-title: Polyhedron doi: 10.1016/0277-5387(94)00329-D contributor: fullname: Basickes |
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