Characteristics and sources of Pb exposure via household dust from the urban area of Shanghai, China

• Published in: The Science of the total environment Vol. 811; p. 151984
• Main Authors: Dong, Chenyin, Liu, Junxia, Harvey, Paul, Yan, Chonghuai
• Format: Journal Article
• Language: English
• Published: Netherlands Elsevier B.V 10.03.2022
• Subjects: air; air quality; Bio-accessibility; blood; Child; childhood; China; coal; combustion; dust; Dust - analysis; environment; Environmental Exposure - analysis; Environmental Monitoring; Exposure risk; gasoline; Humans; Indoor environment; Lead; Lead isotopes; prices; Soil; solid wastes; urban areas; vacuum cleaners; waste incineration; wind speed; China; Lead isotopes; Bio-accessibility; Indoor environment; Exposure risk
• ISSN: 0048-9697; 1879-1026; 1879-1026
• DOI: 10.1016/j.scitotenv.2021.151984

Household dust has been considered as an important pathway for children's environmental Pb exposure. Shanghai was one of the first cities in China that removed Pb from petrol and has been shown in our previous study to have the lowest childhood blood Pb levels in China. This study therefore examines household dust Pb (PbHD) in Shanghai in order to determine the extent and exposure risks of PbHD. Household vacuum cleaner dust samples (n = 40) were collected and analyzed for total Pb concentration, bio-accessible Pb concentration and Pb isotopic compositions (PbIC). The mean concentration of PbHD was 195 mg/kg, which is between 7 and 10 times the Pb concentration of background soil samples from Shanghai. Among the investigated homes, those living in neighborhoods with lower average estate prices have higher dust Pb exposure risks for children. Bio-accessibility of Pb in household dust ranged between 53 and 91%, with a mean value of 71%. Analysis of PbIC of household dust samples (208Pb/206Pb: 2.1096 ± 0.0054; 207Pb/206Pb: 0.8648 ± 0.0025) are a close match to PbIC of coal combustion and solid waste incineration and fit well with those of outdoor air PbIC and urban surface soil PbIC of Shanghai. The study shows that children living in Shanghai are subject to PbHD exposure, with children living in the homes with lower average price having increased susceptibility to PbHD exposure. The data indicate that PbHD is derived primarily from contemporary coal combustion and solid waste incineration rather than common legacy Pb sources (e.g., Pb petrol and paint). Practices including closing doors and windows on days with poor air quality or high wind and preventing shoe wearing inside homes will aid in minimizing outdoor surface soil and ambient particulate intrusion indoors. [Display omitted] •Household dust Pb (PbHD) is elevated compared to background soil from Shanghai.•PbHD in Shanghai is highly bioaccessible with a mean of 71%.•Emissions of coal combustion and solid waste incineration (SWI) are unignorable.•Effects of coal combustion and SWI on PbHD cannot be identified separately.