Experimental investigation of mass efficiency curve for alpha radioactivity counting using a gas-proportional detector

• Published in: Applied radiation and isotopes Vol. 60; no. 6; pp. 879 - 886
• Main Authors: Semkow, T.M., Bari, A., Parekh, P.P., Haines, D.K., Gao, H., Bolden, A.N., Dahms, K.S., Scarpitta, S.C., Thern, R.E., Velazquez, S.
• Format: Journal Article
• Language: English
• Published: England Elsevier Ltd 01.06.2004
• ISSN: 0969-8043; 1872-9800
• DOI: 10.1016/j.apradiso.2004.01.012

Gross α counting of evaporated water residues offers a simple method for screening α radioactivity in water for both public health and emergency purposes. The evaporation process for water has been improved by using a combination of roughening of the surface of counting planchettes, two-stage evaporation, and temperature-controlled block heating. The efficiency of the gas-proportional detector for α-particle detection in water residues was studied as a function of sample mass–thickness in the range between 0.1 and 13 mg cm −2 . The effect of α energy on the efficiency, as well as moisture absorption on the samples, were studied using 230 Th , 238 U , 239 Pu , 241 Am , and 244 Cm radionuclides. Also, α-to- β crosstalk was investigated as a function of sample mass for 230 Th , 239 Pu , 210 Po , 241 Am , and 244 Cm . The improved method can also be applied for gross α detection in biological fluids.