The oxygen reduction activity on platinum-decorated nitrogen-doped bilayer graphene

Studied the oxygen reduction reaction activity of materials with different structures such as single-doped N, single-doped Pt, and double-layer graphene (BLG) co-doped with N and Pt. The BLG models under different doping conditions are established, and then oxygen molecules are adsorbed on the surfa...

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Published inJournal of materials science Vol. 57; no. 4; pp. 2794 - 2802
Main Authors Wang, Ting, Liu, Jianfeng, Miao, Keji, Yin, Yangyang, Ma, Junjie, Yin, Shibin, Pan, Weiguo
Format Journal Article
LanguageEnglish
Published New York Springer US 2022
Springer
Springer Nature B.V
Subjects
Adsorption
Bilayers
Characterization and Evaluation of Materials
Chemistry and Materials Science
Classical Mechanics
Crystallography and Scattering Methods
Doping
Energy Materials
Graphene
Interlayers
Materials Science
Nitrogen
Oxygen reduction reactions
Platinum
Polymer Sciences
Solid Mechanics
Surface chemistry
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Summary:Studied the oxygen reduction reaction activity of materials with different structures such as single-doped N, single-doped Pt, and double-layer graphene (BLG) co-doped with N and Pt. The BLG models under different doping conditions are established, and then oxygen molecules are adsorbed on the surface of BLG-based catalyst models. Through optimizing the structure of established models, the adsorption energy of oxygen for different models is calculated and then compares their oxygen reduction activities. Finally, it is found that the oxygen reduction activity of platinum-decorated and nitrogen-doped BLG is better than that of single doping. Meanwhile, the ORR activity of surface adsorption is also better than that of interlayer adsorption.
ISSN:0022-2461
1573-4803
DOI:10.1007/s10853-021-06677-5