Photothermal control of whispering gallery mode lasing in polymer-coated silica microcavity using high-efficiency nanoheater

Photothermal control has been widely used in the tuning of microelectronic devices due to its laser-assisted noncontact manipulation and cost-effective advantages. The Nd 3+ heavily doped NaGdF 4 nanocrystals (NCs) were proposed as a heat source at nanoscale, and its light-to-heat conversion efficie...

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Bibliographic Details
Published inJournal of materials science Vol. 56; no. 1; pp. 570 - 580
Main Authors Li, Hanyang, Hao, Xiaolei, Li, Yanzeng, Duan, Rui, Zhang, Tingting, Li, Jin, Yuan, Yonggui, Liu, Lu
Format Journal Article
LanguageEnglish
Published New York Springer US 2021
Springer
Springer Nature B.V
Subjects
Characterization and Evaluation of Materials
Chemistry and Materials Science
Classical Mechanics
Continuous radiation
Crystallography and Scattering Methods
Electronic Materials
Lasers
Lasing
Materials Science
Nanocrystals
Photothermal conversion
Polymer coatings
Polymer industry
Polymer Sciences
Polymers
Pulsed lasers
Refractivity
Silica
Silicon dioxide
Solid Mechanics
Tunable lasers
Tuning
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Summary:Photothermal control has been widely used in the tuning of microelectronic devices due to its laser-assisted noncontact manipulation and cost-effective advantages. The Nd 3+ heavily doped NaGdF 4 nanocrystals (NCs) were proposed as a heat source at nanoscale, and its light-to-heat conversion efficiency was evaluated to be above 80%. Here, we obtained a whispering gallery mode lasing emission from the prepared polymer-coated silica microcavity under a 532 nm pulsed laser. The nanoheaters are combined with the microcavity to trigger the photothermal effect at the irradiation of a second 793 nm continuous wave (CW) laser, thereby realizing all-optical tuning of the resonance wavelength by changing the effective refractive index of the microcavity. By measuring the shift of lasing modes on exposure to CW laser with different power intensities, the maximum tuning range and sensitivity of 2 nm and 1.96 nm/(W·mm −2 ) were achieved as the power intensity increased from 0 to 1.02 W/mm 2 . Our work provides a method for developing a new generation of all-optical tunable lasers based on nanoscale photothermal effect. Graphic abstract
ISSN:0022-2461
1573-4803
DOI:10.1007/s10853-020-05272-4