Two-dimensional organic-inorganic hybrid perovskite: from material properties to device applications

• Published in: Science China materials Vol. 61; no. 10; pp. 1257 - 1277
• Main Authors: Ma, Shuang, Cai, Molang, Cheng, Tai, Ding, Xihong, Shi, Xiaoqiang, Alsaedi, Ahmed, Hayat, Tasawar, Ding, Yong, Tan, Zhan’ao, Dai, Songyuan
• Format: Journal Article
• Language: English
• Published: Beijing Science China Press 01.10.2018; Springer Nature B.V
• Subjects: Ammonium halides; Chemistry and Materials Science; Chemistry/Food Science; Light emitting diodes; Material properties; Materials Science; Optoelectronic devices; Organic light emitting diodes; Perovskites; Photovoltaic cells; Reviews; Solar cells; preparation methods; material properties; optoelectronic applications; 2D perovskite
• ISSN: 2095-8226; 2199-4501
• DOI: 10.1007/s40843-018-9294-5

The two-dimensional (2D) perovskite (including pure-2D and quasi-2D) is formed by introducing large-group ammonium halides into conventional bulk perovskite. In the past twenty years, 2D perovskite materials were widely developed with the enriched species and advanced physical-knowledge in material characteristics as well as optoelectronic device applications. To review achievments in 2D perovskite, the fundamental mechanism and properties of 2D perovskite are introduced to offer insight into device performance. Moreover, the preparation methods of 2D perovskite films are summarized and compared. The latest successful applications of the 2D perovskite in the solar cells and light-emitting diodes fields, especially the advanced stability of 2D perovskite solar cells (PeSCs) and the efficient 2D perovskite light-emitting diodes (PeLEDs), are also achieved. Furthermore, the challenges and outlook of 2D perovskite materials are proposed.