Decorating g-C3N4 with alkalinized Ti3C2 MXene for promoted photocatalytic CO2 reduction performance
[Display omitted] Photocatalytic reduction of carbon dioxide (CO2) under visible light irradiation for producing high-value fuel has attracted tremendous attention in recent years. In this study, titanium carbide MXene (Ti3C2) was used as a noble metal-free co-catalyst by simply mixing graphitic car...
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| Published in | Journal of colloid and interface science Vol. 564; pp. 406 - 417 |
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| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier Inc
22.03.2020
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| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
Photocatalytic reduction of carbon dioxide (CO2) under visible light irradiation for producing high-value fuel has attracted tremendous attention in recent years. In this study, titanium carbide MXene (Ti3C2) was used as a noble metal-free co-catalyst by simply mixing graphitic carbon nitride (g-C3N4) and alkalized Ti3C2. The carbon monoxide evolution rate of the optimized composite (5%TCOH-CN) from photocatalytic reduction of CO2 was 5.9 times higher than that of pure g-C3N4. Alkalized Ti3C2 was responsible for the superior photocatalytic activity due to its excellent electrical conductivity and large CO2 adsorption capacity. Furthermore, the separation of the photo-induced electron–hole pairs was greatly enhanced because of the large Fermi level difference between alkalized Ti3C2 and pure g-C3N4. This work demonstrates the potential of MXenes as noble metal-free co-catalyst for photocatalysis processes such as carbon dioxide reduction reaction and nitrogen reduction reaction. |
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| AbstractList | [Display omitted]
Photocatalytic reduction of carbon dioxide (CO2) under visible light irradiation for producing high-value fuel has attracted tremendous attention in recent years. In this study, titanium carbide MXene (Ti3C2) was used as a noble metal-free co-catalyst by simply mixing graphitic carbon nitride (g-C3N4) and alkalized Ti3C2. The carbon monoxide evolution rate of the optimized composite (5%TCOH-CN) from photocatalytic reduction of CO2 was 5.9 times higher than that of pure g-C3N4. Alkalized Ti3C2 was responsible for the superior photocatalytic activity due to its excellent electrical conductivity and large CO2 adsorption capacity. Furthermore, the separation of the photo-induced electron–hole pairs was greatly enhanced because of the large Fermi level difference between alkalized Ti3C2 and pure g-C3N4. This work demonstrates the potential of MXenes as noble metal-free co-catalyst for photocatalysis processes such as carbon dioxide reduction reaction and nitrogen reduction reaction. Photocatalytic reduction of carbon dioxide (CO₂) under visible light irradiation for producing high-value fuel has attracted tremendous attention in recent years. In this study, titanium carbide MXene (Ti₃C₂) was used as a noble metal-free co-catalyst by simply mixing graphitic carbon nitride (g-C₃N₄) and alkalized Ti₃C₂. The carbon monoxide evolution rate of the optimized composite (5%TCOH-CN) from photocatalytic reduction of CO₂ was 5.9 times higher than that of pure g-C₃N₄. Alkalized Ti₃C₂ was responsible for the superior photocatalytic activity due to its excellent electrical conductivity and large CO₂ adsorption capacity. Furthermore, the separation of the photo-induced electron–hole pairs was greatly enhanced because of the large Fermi level difference between alkalized Ti₃C₂ and pure g-C₃N₄. This work demonstrates the potential of MXenes as noble metal-free co-catalyst for photocatalysis processes such as carbon dioxide reduction reaction and nitrogen reduction reaction. Photocatalytic reduction of carbon dioxide (CO2) under visible light irradiation for producing high-value fuel has attracted tremendous attention in recent years. In this study, titanium carbide MXene (Ti3C2) was used as a noble metal-free co-catalyst by simply mixing graphitic carbon nitride (g-C3N4) and alkalized Ti3C2. The carbon monoxide evolution rate of the optimized composite (5%TCOH-CN) from photocatalytic reduction of CO2 was 5.9 times higher than that of pure g-C3N4. Alkalized Ti3C2 was responsible for the superior photocatalytic activity due to its excellent electrical conductivity and large CO2 adsorption capacity. Furthermore, the separation of the photo-induced electron-hole pairs was greatly enhanced because of the large Fermi level difference between alkalized Ti3C2 and pure g-C3N4. This work demonstrates the potential of MXenes as noble metal-free co-catalyst for photocatalysis processes such as carbon dioxide reduction reaction and nitrogen reduction reaction.Photocatalytic reduction of carbon dioxide (CO2) under visible light irradiation for producing high-value fuel has attracted tremendous attention in recent years. In this study, titanium carbide MXene (Ti3C2) was used as a noble metal-free co-catalyst by simply mixing graphitic carbon nitride (g-C3N4) and alkalized Ti3C2. The carbon monoxide evolution rate of the optimized composite (5%TCOH-CN) from photocatalytic reduction of CO2 was 5.9 times higher than that of pure g-C3N4. Alkalized Ti3C2 was responsible for the superior photocatalytic activity due to its excellent electrical conductivity and large CO2 adsorption capacity. Furthermore, the separation of the photo-induced electron-hole pairs was greatly enhanced because of the large Fermi level difference between alkalized Ti3C2 and pure g-C3N4. This work demonstrates the potential of MXenes as noble metal-free co-catalyst for photocatalysis processes such as carbon dioxide reduction reaction and nitrogen reduction reaction. |
| Author | Tang, Qijun Wang, Haiqiang Wu, Zhongbiao Sun, Zhuxing Deng, Shuang |
| Author_xml | – sequence: 1 givenname: Qijun surname: Tang fullname: Tang, Qijun organization: Key Laboratory of Environment Remediation and Ecological Health, Ministry of Education, College of Environmental & Resources Science, Zhejiang University, Hangzhou 310058, PR China – sequence: 2 givenname: Zhuxing surname: Sun fullname: Sun, Zhuxing organization: School of Environmental Science and Engineering, Shanghai Jiao Tong University, Shanghai 200240, PR China – sequence: 3 givenname: Shuang surname: Deng fullname: Deng, Shuang organization: Chinese Research Academy of Environmental Sciences, Beijing 100012, PR China – sequence: 4 givenname: Haiqiang surname: Wang fullname: Wang, Haiqiang email: haiqiangwang@zju.edu.cn organization: Key Laboratory of Environment Remediation and Ecological Health, Ministry of Education, College of Environmental & Resources Science, Zhejiang University, Hangzhou 310058, PR China – sequence: 5 givenname: Zhongbiao surname: Wu fullname: Wu, Zhongbiao organization: Key Laboratory of Environment Remediation and Ecological Health, Ministry of Education, College of Environmental & Resources Science, Zhejiang University, Hangzhou 310058, PR China |
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| Keywords | g-C3N4 Alkalized Ti3C2 Photocatalytic CO2 reduction MXenes |
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Photocatalytic reduction of carbon dioxide (CO2) under visible light irradiation for producing high-value fuel has attracted tremendous... Photocatalytic reduction of carbon dioxide (CO2) under visible light irradiation for producing high-value fuel has attracted tremendous attention in recent... Photocatalytic reduction of carbon dioxide (CO₂) under visible light irradiation for producing high-value fuel has attracted tremendous attention in recent... |
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| SubjectTerms | adsorption Alkalized Ti3C2 carbon dioxide carbon monoxide carbon nitride catalysts electrical conductivity fuels g-C3N4 graphene irradiation light mixing MXenes nitrogen photocatalysis Photocatalytic CO2 reduction titanium |
| Title | Decorating g-C3N4 with alkalinized Ti3C2 MXene for promoted photocatalytic CO2 reduction performance |
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