The photoionization-reduced energy in LSC

• Published in: Applied radiation and isotopes Vol. 64; no. 1; pp. 43 - 54
• Main Authors: Grau Carles, A., Günther, E., Grau Malonda, A.
• Format: Journal Article
• Language: English
• Published: England Elsevier Ltd 2006
• Subjects: Electron-capture; Liquid Scintillation counting; Photoionization; Photoionization; Liquid Scintillation counting; Electron-capture
• ISSN: 0969-8043; 1872-9800
• DOI: 10.1016/j.apradiso.2005.06.005

The atomic rearrangement cascade that follows the electron-capture decay process in low- Z radionuclides involves X-rays which have high photoelectric interaction probabilities. When the K-shell binding energy of the ionized atom (e.g., hydrogen) is significantly lower than the energy of the X-ray photon, the detector response to a photon-equivalent energy electron and the whole photoionization process are very similar. This is not the case when the scintillator cocktail contains larger atoms (e.g., oxygen and phosphorus in Ultima Gold TM ). For larger Z atoms, the reduced energy of the whole photoionization process is less than the reduced energy of the interacting photon due to the nonlinear effects of ionization quenching. This paper shows the convenience of including a more detailed simulation of the photoionization process in the atomic rearrangement detection model for electron-capture nuclides such as 55Fe, 51Cr and 54Mn. The need for more elaborate atomic rearrangement models is a consequence of the analysis of 125I data.