Metal–organic framework-derived porous materials for catalysis
Metal–organic frameworks (MOFs), constructed by metal ions/clusters and organic linkers, featuring crystalline porous structures, have been intensively employed as templates/precursors for the synthesis of diverse porous materials. The large surface area, high porosity and excellent tailorability of...
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| Published in | Coordination chemistry reviews Vol. 362; pp. 1 - 23 |
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| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.05.2018
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Metal–organic frameworks (MOFs), constructed by metal ions/clusters and organic linkers, featuring crystalline porous structures, have been intensively employed as templates/precursors for the synthesis of diverse porous materials. The large surface area, high porosity and excellent tailorability of MOFs can be well inherited to their derivatives, making MOF-derived porous materials very promising for catalytic applications. Herein, we systematically summarize the versatile synthetic strategies to fabricate MOF-derived porous materials and give an overview on their recent progress on heterogeneous organocatalysis, photocatalysis and electrocatalysis. Finally, the challenges and prospects related to MOF-derived porous materials for catalysis are also discussed.
[Display omitted]
•A summary of the versatile synthetic strategies for MOF-derived porous materials.•Recent progress of diverse catalytic reactions over MOF-derived porous materials.•The challenges and prospects related to MOF-derived porous materials for catalysis.
Metal–organic frameworks (MOFs), constructed by metal ions/clusters and organic linkers, featuring crystalline porous structures, have been intensively employed as templates/precursors for the synthesis of diverse porous materials including porous carbons, metal-based compounds (such as metal oxides/carbides/phosphides) and their composites. The large surface area, high porosity and excellent tailorability of MOFs can be well inherited to their derivatives, making MOF-derived porous materials very promising for catalytic applications. Herein, we systematically summarize the versatile synthetic strategies to fabricate MOF-derived porous materials and give an overview on their recent progress on organic heterogeneous catalysis, photocatalysis and electrocatalysis. Finally, the challenges and prospects related to MOF-derived porous materials for catalysis are also discussed. |
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| AbstractList | Metal–organic frameworks (MOFs), constructed by metal ions/clusters and organic linkers, featuring crystalline porous structures, have been intensively employed as templates/precursors for the synthesis of diverse porous materials. The large surface area, high porosity and excellent tailorability of MOFs can be well inherited to their derivatives, making MOF-derived porous materials very promising for catalytic applications. Herein, we systematically summarize the versatile synthetic strategies to fabricate MOF-derived porous materials and give an overview on their recent progress on heterogeneous organocatalysis, photocatalysis and electrocatalysis. Finally, the challenges and prospects related to MOF-derived porous materials for catalysis are also discussed.
[Display omitted]
•A summary of the versatile synthetic strategies for MOF-derived porous materials.•Recent progress of diverse catalytic reactions over MOF-derived porous materials.•The challenges and prospects related to MOF-derived porous materials for catalysis.
Metal–organic frameworks (MOFs), constructed by metal ions/clusters and organic linkers, featuring crystalline porous structures, have been intensively employed as templates/precursors for the synthesis of diverse porous materials including porous carbons, metal-based compounds (such as metal oxides/carbides/phosphides) and their composites. The large surface area, high porosity and excellent tailorability of MOFs can be well inherited to their derivatives, making MOF-derived porous materials very promising for catalytic applications. Herein, we systematically summarize the versatile synthetic strategies to fabricate MOF-derived porous materials and give an overview on their recent progress on organic heterogeneous catalysis, photocatalysis and electrocatalysis. Finally, the challenges and prospects related to MOF-derived porous materials for catalysis are also discussed. |
| Author | Jiao, Long Chen, Yu-Zhen Zhang, Rui Jiang, Hai-Long |
| Author_xml | – sequence: 1 givenname: Yu-Zhen surname: Chen fullname: Chen, Yu-Zhen organization: Hefei National Laboratory for Physical Sciences at the Microscale, CAS Key Laboratory of Soft Matter Chemistry, Collaborative Innovation Center of Suzhou Nano Science and Technology, Department of Chemistry, University of Science and Technology of China, Hefei, Anhui 230026, PR China – sequence: 2 givenname: Rui surname: Zhang fullname: Zhang, Rui organization: Hefei National Laboratory for Physical Sciences at the Microscale, CAS Key Laboratory of Soft Matter Chemistry, Collaborative Innovation Center of Suzhou Nano Science and Technology, Department of Chemistry, University of Science and Technology of China, Hefei, Anhui 230026, PR China – sequence: 3 givenname: Long surname: Jiao fullname: Jiao, Long organization: Hefei National Laboratory for Physical Sciences at the Microscale, CAS Key Laboratory of Soft Matter Chemistry, Collaborative Innovation Center of Suzhou Nano Science and Technology, Department of Chemistry, University of Science and Technology of China, Hefei, Anhui 230026, PR China – sequence: 4 givenname: Hai-Long surname: Jiang fullname: Jiang, Hai-Long email: jianglab@ustc.edu.cn organization: Hefei National Laboratory for Physical Sciences at the Microscale, CAS Key Laboratory of Soft Matter Chemistry, Collaborative Innovation Center of Suzhou Nano Science and Technology, Department of Chemistry, University of Science and Technology of China, Hefei, Anhui 230026, PR China |
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