Atomic ordering and bond relaxation in optical spectra of self-organized InP/GaInP2 Wigner molecule structures
We used transmission electron microscopy, Raman, and photoluminescence spectroscopy to identify the effect of CuPt-type GaP-InP atomic ordering (AO) on the structural and emission properties of self-organized (SO) InP/GaInP2 Wigner molecule (WM) quantum dot (QD) structures. We found that the correla...
Saved in:
Published in | Applied physics letters Vol. 115; no. 20 |
---|---|
Main Authors | , , , , , , , , , , , , , , |
Format | Journal Article |
Language | English |
Published |
11.11.2019
|
Online Access | Get full text |
Cover
Loading…
Summary: | We used transmission electron microscopy, Raman, and photoluminescence spectroscopy to identify the effect of CuPt-type GaP-InP atomic ordering (AO) on the structural and emission properties of self-organized (SO) InP/GaInP2 Wigner molecule (WM) quantum dot (QD) structures. We found that the correlation of AO and SO growth results in the formation of InP/GaInP2 QD/AO-domain (QD/AOD) core-shell composites. This observation shows that intrinsic WMs in this system emerge due to a strong piezoelectric field generated by AODs, which induces QD doping and a built-in magnetic field. We found that the bond relaxation of AODs leads to a decrease in the emission energy of WMs of 80 meV. The photoluminescence spectra of single WMs having an emission energy ∼1.53 eV are presented here, the lowest one reported for this system. |
---|---|
ISSN: | 0003-6951 1077-3118 |
DOI: | 10.1063/1.5126527 |