Improving calibration of forensic glass comparisons by considering uncertainty in feature-based elemental data

• Published in: Chemometrics and intelligent laboratory systems Vol. 217; p. 104399
• Main Authors: Ramos, Daniel, Maroñas, Juan, Almirall, Jose
• Format: Journal Article
• Language: English
• Published: Elsevier B.V 15.10.2021
• Subjects: Forensic glass comparison; Heavy-tailed; LA-ICP-MS; Likelihood ratio; Variational autoencoder; Warped Gaussian mixture; Warped Gaussian mixture; Likelihood ratio; Variational autoencoder; LA-ICP-MS; Heavy-tailed; Forensic glass comparison
• ISSN: 0169-7439; 1873-3239
• DOI: 10.1016/j.chemolab.2021.104399

The computation of likelihood ratios (LR) to measure the weight of forensic glass evidence with LA-ICP-MS data directly in the feature space without computing any kind of score as an intermediate step is a complex problem. A probabilistic two-level modeling of the within-source and between-source variability of the glass samples is needed in order to compare the elemental profiles measured from glass recovered from a suspect or a crime scene and compared to glass samples of a known source of origin. Calibration of the likelihood ratios generated using previously reported models is essential to the realistic reporting of the value of the glass evidence comparisons. We propose models that outperform previously proposed feature-based LR models, in particular by improving the calibration of the computed LRs. We assume that the within-source variability is heavy-tailed, in order to incorporate uncertainty when the available data is scarce, as it typically happens in forensic glass comparison. Moreover, we address the complexity of the between-source variability by the use of probabilistic machine learning algorithms, namely a variational autoencoder and a warped Gaussian mixture. Our results show that the overall performance of the likelihood ratios generated by our model is superior to classical approaches, and that this improvement is due to a dramatic improvement in the calibration despite some loss in discriminating power. Moreover, the robustness of the calibration of our proposal is remarkable. •Forensic glass comparison can be logically and coherently performed by computing a likelihood ratio.•Likelihood ratios coming from forensic comparisons should present good calibration.•We propose the use of a two-level model based on LA-ICP-MS features, with a heavy-tailed within-source variability distribution and complex modeling of the parameter space.•Our proposals dramatically outperform the baseline, presenting objectively acceptable calibration at the cost of some discrimination loss.•Further analysis reveals that the improvement in calibration comes from the incorporation of uncertainty by the heavy-tailed within-source variability distribution.