Interfacing Si‐Based Electrodes: Impact of Liquid Electrolyte and Its Components

As the demand for mobile energy storage devices has steadily increased during the past decades due to the rising popularity of portable electronics as well as the continued implementation of electromobility, energy density has become a crucial metric in the development of modern batteries. It was re...

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Published inAdvanced materials interfaces Vol. 9; no. 8
Main Authors Wölke, Christian, Sadeghi, Bahareh A., Eshetu, Gebrekidan G., Figgemeier, Egbert, Winter, Martin, Cekic‐Laskovic, Isidora
Format Journal Article
LanguageEnglish
Published Weinheim John Wiley & Sons, Inc 01.03.2022
Subjects
Electrode materials
Electrodes
Electrolytes
Energy storage
Flux density
functional additives
Lithium
lithium salt
Lithium-ion batteries
Silicon
silicon electrode
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Abstract As the demand for mobile energy storage devices has steadily increased during the past decades due to the rising popularity of portable electronics as well as the continued implementation of electromobility, energy density has become a crucial metric in the development of modern batteries. It was realized early on that the successful utilization of silicon as negative electrode material in lithium‐ion batteries would be a quantum leap in improving achievable energy densities due to the roughly ten‐fold increase in specific capacity compared to the state‐of‐the‐art graphite material. However, being an alloying type material rather than an intercalation/insertion type, silicon poses numerous obstacles that need to be overcome for its successful implementation as a negative electrode material with the most prominent one being its extreme volume changes on (de‐)lithiation. While, as of today, a plethora of different types of Si‐based electrodes have been reported, a universally common feature is the interface between Si‐based electrode and electrolyte. This review focuses on the knowledge gained thus far on the impact of different liquid electrolyte components/formulations on the interfaces and interphases encountered at Si‐based electrodes. Silicon‐based electrodes are in the focus of numerous research endeavors aiming at increasing the energy density of lithium‐ion batteries. Overcoming the imposed challenges around silicon as negative electrode, addresses tailoring of electrolyte formulation(s). This work highlights wide variety of different compounds used as electrolyte solvents/co‐solvents, conducting salts and additives and summarizes their impact on the interphases formed on silicon‐based electrodes.
AbstractList Abstract As the demand for mobile energy storage devices has steadily increased during the past decades due to the rising popularity of portable electronics as well as the continued implementation of electromobility, energy density has become a crucial metric in the development of modern batteries. It was realized early on that the successful utilization of silicon as negative electrode material in lithium‐ion batteries would be a quantum leap in improving achievable energy densities due to the roughly ten‐fold increase in specific capacity compared to the state‐of‐the‐art graphite material. However, being an alloying type material rather than an intercalation/insertion type, silicon poses numerous obstacles that need to be overcome for its successful implementation as a negative electrode material with the most prominent one being its extreme volume changes on (de‐)lithiation. While, as of today, a plethora of different types of Si‐based electrodes have been reported, a universally common feature is the interface between Si‐based electrode and electrolyte. This review focuses on the knowledge gained thus far on the impact of different liquid electrolyte components/formulations on the interfaces and interphases encountered at Si‐based electrodes.
As the demand for mobile energy storage devices has steadily increased during the past decades due to the rising popularity of portable electronics as well as the continued implementation of electromobility, energy density has become a crucial metric in the development of modern batteries. It was realized early on that the successful utilization of silicon as negative electrode material in lithium‐ion batteries would be a quantum leap in improving achievable energy densities due to the roughly ten‐fold increase in specific capacity compared to the state‐of‐the‐art graphite material. However, being an alloying type material rather than an intercalation/insertion type, silicon poses numerous obstacles that need to be overcome for its successful implementation as a negative electrode material with the most prominent one being its extreme volume changes on (de‐)lithiation. While, as of today, a plethora of different types of Si‐based electrodes have been reported, a universally common feature is the interface between Si‐based electrode and electrolyte. This review focuses on the knowledge gained thus far on the impact of different liquid electrolyte components/formulations on the interfaces and interphases encountered at Si‐based electrodes.
As the demand for mobile energy storage devices has steadily increased during the past decades due to the rising popularity of portable electronics as well as the continued implementation of electromobility, energy density has become a crucial metric in the development of modern batteries. It was realized early on that the successful utilization of silicon as negative electrode material in lithium‐ion batteries would be a quantum leap in improving achievable energy densities due to the roughly ten‐fold increase in specific capacity compared to the state‐of‐the‐art graphite material. However, being an alloying type material rather than an intercalation/insertion type, silicon poses numerous obstacles that need to be overcome for its successful implementation as a negative electrode material with the most prominent one being its extreme volume changes on (de‐)lithiation. While, as of today, a plethora of different types of Si‐based electrodes have been reported, a universally common feature is the interface between Si‐based electrode and electrolyte. This review focuses on the knowledge gained thus far on the impact of different liquid electrolyte components/formulations on the interfaces and interphases encountered at Si‐based electrodes. Silicon‐based electrodes are in the focus of numerous research endeavors aiming at increasing the energy density of lithium‐ion batteries. Overcoming the imposed challenges around silicon as negative electrode, addresses tailoring of electrolyte formulation(s). This work highlights wide variety of different compounds used as electrolyte solvents/co‐solvents, conducting salts and additives and summarizes their impact on the interphases formed on silicon‐based electrodes.
Author Sadeghi, Bahareh A.
Cekic‐Laskovic, Isidora
Figgemeier, Egbert
Wölke, Christian
Eshetu, Gebrekidan G.
Winter, Martin
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  givenname: Gebrekidan G.
  surname: Eshetu
  fullname: Eshetu, Gebrekidan G.
  organization: RWTH Aachen University
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  surname: Figgemeier
  fullname: Figgemeier, Egbert
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  surname: Winter
  fullname: Winter, Martin
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  givenname: Isidora
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  surname: Cekic‐Laskovic
  fullname: Cekic‐Laskovic, Isidora
  email: i.cekic-laskovic@fz-juelich.de
  organization: Helmholtz‐Institute Münster (IEK‐12)
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Snippet As the demand for mobile energy storage devices has steadily increased during the past decades due to the rising popularity of portable electronics as well as...
Abstract As the demand for mobile energy storage devices has steadily increased during the past decades due to the rising popularity of portable electronics as...
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SubjectTerms Electrode materials
Electrodes
Electrolytes
Energy storage
Flux density
functional additives
Lithium
lithium salt
Lithium-ion batteries
Silicon
silicon electrode
Title Interfacing Si‐Based Electrodes: Impact of Liquid Electrolyte and Its Components
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fadmi.202101898
https://www.proquest.com/docview/2638161466
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