Reconstruction of attosecond pulses in the presence of interfering dressing fields using a 100 kHz laser system at ELI-ALPS

Attosecond Pulse Trains (APT) generated by high-harmonic generation (HHG) of high-intensity near-infrared (IR) laser pulses have proven valuable for studying the electronic dynamics of atomic and molecular species. However, the high intensities required for high-photon-energy, high-flux HHG usually...

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Published inJournal of physics. B, Atomic, molecular, and optical physics Vol. 52; no. 23; pp. 23 - 29
Main Authors Hammerland, D, Zhang, P, Kühn, S, Jojart, P, Seres, I, Zuba, V, Varallyay, Z, Charalambidis, D, Osvay, K, Luu, T T, Wörner, H J
Format Journal Article
LanguageEnglish
Published IOP Publishing 14.12.2019
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Summary:Attosecond Pulse Trains (APT) generated by high-harmonic generation (HHG) of high-intensity near-infrared (IR) laser pulses have proven valuable for studying the electronic dynamics of atomic and molecular species. However, the high intensities required for high-photon-energy, high-flux HHG usually limit the class of adequate laser systems to repetition rates below 10 kHz. Here, APT's generated from the 100 kHz, 160 W, 40 fs laser system (HR-1) currently under commissioning at the extreme light infrastructure attosecond light pulse source (ELI-ALPS) are reconstructed using the reconstruction of attosecond beating by interference of two-photon Transitions (RABBIT) technique. These experiments constitute the first attosecond time-resolved photoelectron spectroscopy measurements with attosecond pulses performed at 100 kHz repetition rate and one of the first experiments performed at ELI-ALPS in the framework of projects commissioning its newly installed technologies. These RABBIT measurements were taken with an additional IR field temporally locked to the extreme-ultraviolet APT, resulting in an atypical beating. We show that the phase of the 2 beating recorded under these conditions is strictly identical to that observed in standard RABBIT measurements within second-order perturbation theory. This work highlights an experimental simplification for future experiments based on attosecond interferometry (or RABBIT), which is particularly useful when lasers with high average powers are used.
Bibliography:JPHYSB-105462.R2
ISSN:0953-4075
1361-6455
DOI:10.1088/1361-6455/ab486c