Pd-Ru nanocatalysts derived from a Pd-induced aerogel for dramatic boosting of hydrogen release

Alloyed bimetallic Pd-Ru nanocatalysts prepared by in situ reduction of a mixture of a Ru(iii) source and a Pd(ii)@alkyne-PVA aerogel and characterized by TEM and XPS exhibit very highly catalytic activity towards hydrogen release from ammonia borane hydrolysis with a TOF value of 578.2 mol mol min...

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Published inNanoscale Vol. 12; no. 4; pp. 2345 - 2349
Main Authors Yang, Xiaojiao, Wei, Jianyu, Wang, Qi, Shuai, Maobing, Yue, Guozong, Li, Peilong, Huang, Deshun, Astruc, Didier, Zhao, Pengxiang
Format Journal Article
LanguageEnglish
Published England Royal Society of Chemistry 28.01.2020
Subjects
Aerogels
Alkynes
Alloying
Ammonia
Bimetals
Catalytic activity
Ruthenium
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Summary:Alloyed bimetallic Pd-Ru nanocatalysts prepared by in situ reduction of a mixture of a Ru(iii) source and a Pd(ii)@alkyne-PVA aerogel and characterized by TEM and XPS exhibit very highly catalytic activity towards hydrogen release from ammonia borane hydrolysis with a TOF value of 578.2 mol mol min .
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ISSN:2040-3364
2040-3372
DOI:10.1039/c9nr09307a