Optical properties of monolayer transition metal dichalcogenides probed by spectroscopic ellipsometry

Spectroscopic ellipsometry was used to characterize the complex refractive index of chemical-vapor-deposited monolayer transition metal dichalcogenides (TMDs). The extraordinary large value of the refractive index in the visible frequency range is obtained. The absorption response shows a strong cor...

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Published inApplied physics letters Vol. 105; no. 20
Main Authors Liu, Hsiang-Lin, Shen, Chih-Chiang, Su, Sheng-Han, Hsu, Chang-Lung, Li, Ming-Yang, Li, Lain-Jong
Format Journal Article
LanguageEnglish
Published Melville American Institute of Physics 17.11.2014
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Abstract Spectroscopic ellipsometry was used to characterize the complex refractive index of chemical-vapor-deposited monolayer transition metal dichalcogenides (TMDs). The extraordinary large value of the refractive index in the visible frequency range is obtained. The absorption response shows a strong correlation between the magnitude of the exciton binding energy and band gap energy. Together with the observed giant spin-orbit splitting, these findings advance the fundamental understanding of their novel electronic structures and the development of monolayer TMDs-based optoelectronic and spintronic devices.
AbstractList Spectroscopic ellipsometry was used to characterize the complex refractive index of chemical-vapor-deposited monolayer transition metal dichalcogenides (TMDs). The extraordinary large value of the refractive index in the visible frequency range is obtained. The absorption response shows a strong correlation between the magnitude of the exciton binding energy and band gap energy. Together with the observed giant spin-orbit splitting, these findings advance the fundamental understanding of their novel electronic structures and the development of monolayer TMDs-based optoelectronic and spintronic devices.
Author Liu, Hsiang-Lin
Li, Lain-Jong
Su, Sheng-Han
Shen, Chih-Chiang
Li, Ming-Yang
Hsu, Chang-Lung
Author_xml – sequence: 1
  givenname: Hsiang-Lin
  surname: Liu
  fullname: Liu, Hsiang-Lin
– sequence: 2
  givenname: Chih-Chiang
  surname: Shen
  fullname: Shen, Chih-Chiang
– sequence: 3
  givenname: Sheng-Han
  surname: Su
  fullname: Su, Sheng-Han
– sequence: 4
  givenname: Chang-Lung
  surname: Hsu
  fullname: Hsu, Chang-Lung
– sequence: 5
  givenname: Ming-Yang
  surname: Li
  fullname: Li, Ming-Yang
– sequence: 6
  givenname: Lain-Jong
  surname: Li
  fullname: Li, Lain-Jong
BackLink https://www.osti.gov/biblio/22391998$$D View this record in Osti.gov
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Snippet Spectroscopic ellipsometry was used to characterize the complex refractive index of chemical-vapor-deposited monolayer transition metal dichalcogenides (TMDs)....
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SubjectTerms Applied physics
BINDING ENERGY
CHALCOGENIDES
CHEMICAL VAPOR DEPOSITION
CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY
ELECTRONIC STRUCTURE
ELLIPSOMETRY
Energy gap
L-S COUPLING
Monolayers
Optical properties
OPTOELECTRONIC DEVICES
Organic chemistry
REFRACTIVE INDEX
Refractivity
Spectroellipsometry
Spectroscopy
TRANSITION ELEMENTS
Transition metal compounds
Title Optical properties of monolayer transition metal dichalcogenides probed by spectroscopic ellipsometry
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https://www.osti.gov/biblio/22391998
Volume 105
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