Measurement of the absolute gamma emission intensities from the decay of Th-229 in equilibrium with progeny

• Published in: Applied radiation and isotopes Vol. 166; p. 109323
• Main Authors: Gomes, R.S., Delgado, J.U., da Silva, C.J., da Silva, R.L., da Cruz, P.A.L., Ferreira Filho, A.L., de Almeida, M.C.M., Iwahara, A., de Oliveira, A.E., Tauhata, L.
• Format: Journal Article
• Language: English
• Published: Elsevier Ltd 01.12.2020
• Subjects: Anticoincidence counting; Gamma emission intensities; Primary standardization; Th-229; γ-ray spectrometry; γ-ray spectrometry; Primary standardization; Th-229; Anticoincidence counting; Gamma emission intensities
• ISSN: 0969-8043; 1872-9800
• DOI: 10.1016/j.apradiso.2020.109323

There are few long-lived radionuclides yielding high intensity gamma-rays emission with energies ranging from 100 keV to 500 keV that can be applied as radioactive gamma standard to calibrate HPGe detectors. Furthermore, this energy range represents the main emitted energies of the majority of radionuclides used in nuclear medicine. The Brazilian National Laboratory for Ionizing Radiation Metrology (LNMRI/IRD/CNEN) has attempted to identify radionuclides that have the potential to be used as a calibration source due to their long half-life as well as their emission spectrum. Hence, LNMRI promotes standardization studies of gamma-emitting radionuclides that meet these criteria on order to disseminate them. Thorium-229, with its well-defined energies and relatively high intensities, is one such candidate radionuclide for the energy and full-energy peak efficiency calibration of high-purity gamma spectrometers. Thorium-229 was standardized by the method of 4παβ(LS)-γ(NaI(Tl)) live timed anticoincidence counting. The emission intensities of gamma-rays associated with the decay of 229Th have been determined by HPGe gamma ray spectrometry with accuracy and precision. The results are in agreement with current literature data. •229Th was standardized by anticoincidence counting system.•The gamma-ray emission intensities of 229Th was determined with a High Purity Germanium (HPGe) detector.•The gamma-ray emission intensities measured are consistent with literature values.