A multijunction of ZnIn2S4 nanosheet/TiO2 film/Si nanowire for significant performance enhancement of water splitting
Photoelectrodes with a specific structure and composition have been proposed for improving the efficiency of solar water splitting. Here, a novel multijunction structure was fabricated, with Si nanowires as cores, ZnIn2S4 nanosheets as branches, and TiO2 films as sandwiched layers. This junction exh...
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| Published in | Nano research Vol. 8; no. 11; pp. 3524 - 3534 |
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| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Beijing
Tsinghua University Press
01.11.2015
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Photoelectrodes with a specific structure and composition have been proposed for improving the efficiency of solar water splitting. Here, a novel multijunction structure was fabricated, with Si nanowires as cores, ZnIn2S4 nanosheets as branches, and TiO2 films as sandwiched layers. This junction exhibited a superior photoelectrochemical performance with a maximum photoconversion efficiency of 0.51%, which is 795 and 64 times higher than that of a bare Si wafer and nanowires, respectively. The large enhancement was attributed to the effective electron-hole separation and fast excited carrier transport within the multijunctions resulting from their favorable energy band alignments with water redox potentials, and to the enlarged contact area for facilitating the electron transfer at the multijunction/electrolyte interface. |
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| AbstractList | Photoelectrodes with a specific structure and composition have been proposed for improving the efficiency of solar water splitting. Here, a novel multijunction structure was fabricated, with Si nanowires as cores, ZnIn2S4 nanosheets as branches, and TiO2 films as sandwiched layers. This junction exhibited a superior photoelectrochemical performance with a maximum photoconversion efficiency of 0.51%, which is 795 and 64 times higher than that of a bare Si wafer and nanowires, respectively. The large enhancement was attributed to the effective electron–hole separation and fast excited carrier transport within the multijunctions resulting from their favorable energy band alignments with water redox potentials, and to the enlarged contact area for facilitating the electron transfer at the multijunction/electrolyte interface. Photoelectrodes with a specific structure and composition have been proposed for improving the efficiency of solar water splitting. Here, a novel multijunction structure was fabricated, with Si nanowires as cores, ZnIn 2 S 4 nanosheets as branches, and TiO 2 films as sandwiched layers. This junction exhibited a superior photoelectrochemical performance with a maximum photoconversion efficiency of 0.51%, which is 795 and 64 times higher than that of a bare Si wafer and nanowires, respectively. The large enhancement was attributed to the effective electron–hole separation and fast excited carrier transport within the multijunctions resulting from their favorable energy band alignments with water redox potentials, and to the enlarged contact area for facilitating the electron transfer at the multijunction/electrolyte interface. |
| Author | Qiong Liu Fangli Wu Fengren Cao Lei Chen Xinjian Xie Weichao Wang Wei Tian Liang Li |
| AuthorAffiliation | College of Physics, Optoelectronics and Energy, Jiangsu Key Laboratory of Thin Films, Soochow University, Suzhou 215006, China Department of Electronics, Tianjin Key Laborotory of Photo-Electronic Thin Film Device and Technology, Nankai University, Tianjin 370001, China |
| Author_xml | – sequence: 1 givenname: Qiong surname: Liu fullname: Liu, Qiong organization: College of Physics, Optoelectronics and Energy, Jiangsu Key Laboratory of Thin Films, Soochow University – sequence: 2 givenname: Fangli surname: Wu fullname: Wu, Fangli organization: College of Physics, Optoelectronics and Energy, Jiangsu Key Laboratory of Thin Films, Soochow University – sequence: 3 givenname: Fengren surname: Cao fullname: Cao, Fengren organization: College of Physics, Optoelectronics and Energy, Jiangsu Key Laboratory of Thin Films, Soochow University – sequence: 4 givenname: Lei surname: Chen fullname: Chen, Lei organization: Department of Electronics, Tianjin Key Laboratory of Photo-Electronic Thin Film Device and Technology, Nankai University – sequence: 5 givenname: Xinjian surname: Xie fullname: Xie, Xinjian organization: Department of Electronics, Tianjin Key Laboratory of Photo-Electronic Thin Film Device and Technology, Nankai University – sequence: 6 givenname: Weichao surname: Wang fullname: Wang, Weichao organization: Department of Electronics, Tianjin Key Laboratory of Photo-Electronic Thin Film Device and Technology, Nankai University – sequence: 7 givenname: Wei surname: Tian fullname: Tian, Wei email: wtian@suda.edu.cn organization: College of Physics, Optoelectronics and Energy, Jiangsu Key Laboratory of Thin Films, Soochow University – sequence: 8 givenname: Liang surname: Li fullname: Li, Liang email: lli@suda.edu.cn organization: College of Physics, Optoelectronics and Energy, Jiangsu Key Laboratory of Thin Films, Soochow University |
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| Copyright | Tsinghua University Press and Springer-Verlag Berlin Heidelberg 2015 Nano Research is a copyright of Springer, (2015). All Rights Reserved. |
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| Notes | 11-5974/O4 Photoelectrodes with a specific structure and composition have been proposed for improving the efficiency of solar water splitting. Here, a novel multijunction structure was fabricated, with Si nanowires as cores, ZnIn2S4 nanosheets as branches, and TiO2 films as sandwiched layers. This junction exhibited a superior photoelectrochemical performance with a maximum photoconversion efficiency of 0.51%, which is 795 and 64 times higher than that of a bare Si wafer and nanowires, respectively. The large enhancement was attributed to the effective electron-hole separation and fast excited carrier transport within the multijunctions resulting from their favorable energy band alignments with water redox potentials, and to the enlarged contact area for facilitating the electron transfer at the multijunction/electrolyte interface. water splitting, photoelectrochemical cells, nanosheets, atomic layer deposition, multi junction ObjectType-Article-1 SourceType-Scholarly Journals-1 ObjectType-Feature-2 content type line 14 |
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| SubjectTerms | Atomic/Molecular Structure and Spectra Biomedicine Biotechnology Carrier transport Chemistry and Materials Science Condensed Matter Physics Electron transfer Materials Science Nanosheets Nanotechnology Nanowires Performance enhancement Quantum efficiency Research Article Silicon Splitting TiO2 Titanium dioxide Water splitting 光解水 增强膜 多结 性能 氧化还原电位 硅纳米线 载流子输运 |
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| Title | A multijunction of ZnIn2S4 nanosheet/TiO2 film/Si nanowire for significant performance enhancement of water splitting |
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