Microbubble generation with rapid dissolution of ammonia (NH3)-hydrogen (H2) mixed gas fed from a nozzle into water

• Published in: Chemical engineering science Vol. 248; p. 117155
• Main Authors: Kobayashi, Taro, Fujioka, Satoko, Tanaka, Shunya, Terasaka, Koichi
• Format: Journal Article
• Language: English
• Published: Elsevier Ltd 02.02.2022
• Subjects: Ammonia gas; Gas dissolution; Hydrogen; Microbubble; Microbubble; Gas dissolution; Ammonia gas; Hydrogen
• ISSN: 0009-2509; 1873-4405
• DOI: 10.1016/j.ces.2021.117155

•Generation of microbubbles has succeeded by the fast dissolution of ammonia gas.•Bubble formation behavior was investigated by using an ultrahigh-speed camera.•Microbubbles were generated by the crushing of the primary bubble.•Distributed microbubble size was affected by the ammonia concentration in liquid.•Increasing of superficial gas velocity decreased microbubbles diameter. Because of their useful characteristics, microbubbles attracted much interest in industry and medicine. In this study, we developed a novel method of generating microbubbles through the chemical absorption of ammonia (NH3). By using an ultrahigh-speed camera, consecutive images of bubble formation were captured, and the microbubble generation mechanism was investigated. The effects of the gas flow rate and ammonia concentration in the liquid phase on the size of the microbubbles were examined. The hydrogen (H2) gas flow rate was found not to demonstrate a significant effect on the bubble diameter. The diameter of the microbubbles increased as the superficial velocity of the gas mixture (NH3 – H2) decreased.