Vapour phase tert-butylation of naphthalene over molecular sieve catalysts
The vapour phase tert-butylation of naphthalene was carried out over modified Y, MCM-41 and SAPO-5 catalysts. CeY was found to be better catalyst among the catalysts screened for this reaction at 200 °C reaction temperature and 0.5 h −1 weight hourly space velocity (WHSV). Various reaction parameter...
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Published in | Microporous and mesoporous materials Vol. 52; no. 3; pp. 151 - 158 |
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Main Authors | , , , |
Format | Journal Article |
Language | English |
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01.05.2002
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Abstract | The vapour phase
tert-butylation of naphthalene was carried out over modified Y, MCM-41 and SAPO-5 catalysts. CeY was found to be better catalyst among the catalysts screened for this reaction at 200 °C reaction temperature and 0.5 h
−1 weight hourly space velocity (WHSV). Various reaction parameters like reaction temperature, mole ratio, WHSV and time on stream were studied for this reaction. Acidity of the catalysts was determined using stepwise temperature programmed desorption (STPD) technique and correlated to the product selectivity. Attempt has been made to explain the shape selectivity of catalyst and the product selectivity. |
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AbstractList | The vapour phase
tert-butylation of naphthalene was carried out over modified Y, MCM-41 and SAPO-5 catalysts. CeY was found to be better catalyst among the catalysts screened for this reaction at 200 °C reaction temperature and 0.5 h
−1 weight hourly space velocity (WHSV). Various reaction parameters like reaction temperature, mole ratio, WHSV and time on stream were studied for this reaction. Acidity of the catalysts was determined using stepwise temperature programmed desorption (STPD) technique and correlated to the product selectivity. Attempt has been made to explain the shape selectivity of catalyst and the product selectivity. |
Author | Kulkarni, S.J. Raghavan, K.V. Kamalakar, G. Prasad, M.Ramakrishna |
Author_xml | – sequence: 1 givenname: G. surname: Kamalakar fullname: Kamalakar, G. – sequence: 2 givenname: M.Ramakrishna surname: Prasad fullname: Prasad, M.Ramakrishna – sequence: 3 givenname: S.J. surname: Kulkarni fullname: Kulkarni, S.J. email: sjkulkarni@iict.ap.nic.in – sequence: 4 givenname: K.V. surname: Raghavan fullname: Raghavan, K.V. |
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Keywords | Butylation Acidity Naphthalene mono- tert-butylnaphthalene (MTBN) di- tert-butylnaphthalene (DTBN) Catalytic reaction Catalyst selectivity Acidic site Modified catalyst Zeolite Experimental study Alkylation Molecular sieve Heterogeneous catalysis Iron ion Tertiary alcohol Preparation Butanol Cerium ion Hydrothermal condition |
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tert-butylation of naphthalene was carried out over modified Y, MCM-41 and SAPO-5 catalysts. CeY was found to be better catalyst among the... |
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SubjectTerms | Acidity Butylation Catalysis Catalytic reactions Chemistry di- tert-butylnaphthalene (DTBN) Exact sciences and technology General and physical chemistry mono- tert-butylnaphthalene (MTBN) Naphthalene Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry |
Title | Vapour phase tert-butylation of naphthalene over molecular sieve catalysts |
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