Pd/Lewis Acid Synergy in Macroporous Pd@Na‐ZSM‐5 for Enhancing Selective Conversion of Biomass

Pd nanometal particles encapsulated in macroporous Na‐ZSM‐5 with only Lewis acid sites have been successfully synthesized by a steam‐thermal approach. The synergistic effect of Pd and Lewis acid sites have been investigated for significant enhancement of the catalytic selectivity towards furfural al...

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Published inChemCatChem Vol. 12; no. 21; pp. 5364 - 5368
Main Authors Liu, Jia‐Wen, Wu, Si‐Ming, Wang, Li‐Ying, Tian, Ge, Qin, Yuan, Wu, Jing‐Xian, Zhao, Xiao‐Fang, Zhang, Yan‐Xiang, Chang, Gang‐Gang, Wu, Lu, Zhang, Yue‐Xing, Li, Zhao‐Fei, Guo, Cheng‐Yu, Janiak, Christoph, Lenaerts, Silvia, Yang, Xiao‐Yu
Format Journal Article
LanguageEnglish
Published 05.11.2020
Subjects
biomass conversion
confinement effect
Lewis acids
Pd cluster
synergistic effect
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Summary:Pd nanometal particles encapsulated in macroporous Na‐ZSM‐5 with only Lewis acid sites have been successfully synthesized by a steam‐thermal approach. The synergistic effect of Pd and Lewis acid sites have been investigated for significant enhancement of the catalytic selectivity towards furfural alcohol in furfural hydroconversion. Confinement effect: The synergy effect of Pd and Lewis acid sites confined in Pd@macroporous Na‐ZSM‐5 significantly enhance the catalytic selectivity in biomass conversion.
Bibliography:These authors contributed equally to this work.
ISSN:1867-3880
1867-3899
DOI:10.1002/cctc.202000868