Difference in magnetic properties and magnetocaloric effect of FeRh0.98Al0.02 alloy with different sample sizes
•The flake sample with smaller particles of FeRh0.98Al0.02 alloy undergoes a more pronounced first-order AFM-FM transition than the chunk sample.•The flake and chunk of FeRh0.98Al0.02 alloy exhibit different AFM-FM phase transition temperature and thermal hysteresis.•The chunk FeRh0.98Al0.02 alloy d...
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| Published in | Journal of magnetism and magnetic materials Vol. 535; p. 168034 |
|---|---|
| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
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Amsterdam
Elsevier B.V
01.10.2021
Elsevier BV |
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| Abstract | •The flake sample with smaller particles of FeRh0.98Al0.02 alloy undergoes a more pronounced first-order AFM-FM transition than the chunk sample.•The flake and chunk of FeRh0.98Al0.02 alloy exhibit different AFM-FM phase transition temperature and thermal hysteresis.•The chunk FeRh0.98Al0.02 alloy displays magnetocaloric properties suitable for magnetic refrigeration near room temperature.•The chunk sample exhibits 54% larger RC value compared to flakes.
Magnetic and magnetocaloric properties of the polycrystalline FeRh0.98Al0.02 alloy have been investigated as function of its physical state. A flake FeRh0.98Al0.02 sample undergoes an antiferromagnetic (AFM)-ferromagnetic (FM) phase transition around 275 K during heating and displays a 20 K thermal hysteresis upon the following cooling with an applied field of 5kOe. However, for a solid chunk sample, the transition temperature is around 308 K on heating and the hysteresis is 16 K. The maximum magnetic entropy change (ΔSM) is 3.1 and 2.7 J/kg K for μ0ΔH = 30 kOe and the refrigerant capacity (RC) is 120 and 185 J/kg for the flake and chunk samples, respectively. The temperature of the ΔSM maximum for the flake samples changes for different values of ΔH, which is characteristic for a first-order transition. On the other hand, the temperature remains almost constant for the chunk sample. |
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| AbstractList | Magnetic and magnetocaloric properties of the polycrystalline FeRh0.98Al0.02 alloy have been investigated as function of its physical state. A flake FeRh0.98Al0.02 sample undergoes an antiferromagnetic (AFM)-ferromagnetic (FM) phase transition around 275 K during heating and displays a 20 K thermal hysteresis upon the following cooling with an applied field of 5 kOe. However, for a solid chunk sample, the transition temperature is around 308 K on heating and the hysteresis is 16 K. The maximum magnetic entropy change (ΔSM) is 3.1 and 2.7 J/kg K for μ0ΔH = 30 kOe and the refrigerant capacity (RC) is 120 and 185 J/kg for the flake and chunk samples, respectively. The temperature of the ΔSM maximum for the flake samples changes for different values of ΔH, which is characteristic for a first-order transition. On the other hand, the temperature remains almost constant for the chunk sample. •The flake sample with smaller particles of FeRh0.98Al0.02 alloy undergoes a more pronounced first-order AFM-FM transition than the chunk sample.•The flake and chunk of FeRh0.98Al0.02 alloy exhibit different AFM-FM phase transition temperature and thermal hysteresis.•The chunk FeRh0.98Al0.02 alloy displays magnetocaloric properties suitable for magnetic refrigeration near room temperature.•The chunk sample exhibits 54% larger RC value compared to flakes. Magnetic and magnetocaloric properties of the polycrystalline FeRh0.98Al0.02 alloy have been investigated as function of its physical state. A flake FeRh0.98Al0.02 sample undergoes an antiferromagnetic (AFM)-ferromagnetic (FM) phase transition around 275 K during heating and displays a 20 K thermal hysteresis upon the following cooling with an applied field of 5kOe. However, for a solid chunk sample, the transition temperature is around 308 K on heating and the hysteresis is 16 K. The maximum magnetic entropy change (ΔSM) is 3.1 and 2.7 J/kg K for μ0ΔH = 30 kOe and the refrigerant capacity (RC) is 120 and 185 J/kg for the flake and chunk samples, respectively. The temperature of the ΔSM maximum for the flake samples changes for different values of ΔH, which is characteristic for a first-order transition. On the other hand, the temperature remains almost constant for the chunk sample. |
| ArticleNumber | 168034 |
| Author | Shang, Yafen Li, Yanzhuo Zhou, Xiaoyu Fu, Hao Mozharivskyj, Yurij |
| Author_xml | – sequence: 1 givenname: Yafen surname: Shang fullname: Shang, Yafen organization: School of Physics, University of Electronic Science and Technology of China, Chengdu 611731, People’s Republic of China – sequence: 2 givenname: Xiaoyu surname: Zhou fullname: Zhou, Xiaoyu organization: School of Physics, University of Electronic Science and Technology of China, Chengdu 611731, People’s Republic of China – sequence: 3 givenname: Yanzhuo surname: Li fullname: Li, Yanzhuo organization: School of Physics, University of Electronic Science and Technology of China, Chengdu 611731, People’s Republic of China – sequence: 4 givenname: Yurij surname: Mozharivskyj fullname: Mozharivskyj, Yurij organization: Department of Chemistry and Chemical Biology, Brockhouse Institute of Materials Research, McMaster University, 1280 Main Street West, Hamilton, Ontario L8S 4M1, Canada – sequence: 5 givenname: Hao surname: Fu fullname: Fu, Hao email: fuhao@uestc.edu.cn organization: School of Physics, University of Electronic Science and Technology of China, Chengdu 611731, People’s Republic of China |
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| Snippet | •The flake sample with smaller particles of FeRh0.98Al0.02 alloy undergoes a more pronounced first-order AFM-FM transition than the chunk sample.•The flake and... Magnetic and magnetocaloric properties of the polycrystalline FeRh0.98Al0.02 alloy have been investigated as function of its physical state. A flake... |
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| SubjectTerms | Antiferromagnetism Ferromagnetism Flakes Heating Hysteresis Magnetic entropy change Magnetic properties Magnetic refrigeration Magnetism Magnetocaloric effect Phase transition Phase transitions Transition temperature |
| Title | Difference in magnetic properties and magnetocaloric effect of FeRh0.98Al0.02 alloy with different sample sizes |
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