A Reusable Cobalt Catalyst for Reversible Acceptorless Dehydrogenation and Hydrogenation of N‐Heterocycles

The development of robust catalytic systems based on base‐metals for reversible acceptorless dehydrogenation (ADH) and hydrogenation of feedstock chemicals is very important in the context of ‘hydrogen storage’. Herein, we report a highly efficient reusable cobalt‐based heterogeneous catalyst for re...

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Bibliographic Details
Published inChemCatChem Vol. 11; no. 10; pp. 2449 - 2457
Main Authors Jaiswal, Garima, Subaramanian, Murugan, Sahoo, Manoj K., Balaraman, Ekambaram
Format Journal Article
LanguageEnglish
Published Weinheim Wiley Subscription Services, Inc 20.05.2019
Subjects
Acceptorless dehydrogenation
Catalysis
Catalysts
Cobalt
Cobalt catalyst
Dehydrogenation
Heterogeneous catalysis
Hydrogen storage
Hydrogenation
N-heterocycles
Organic chemistry
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Summary:The development of robust catalytic systems based on base‐metals for reversible acceptorless dehydrogenation (ADH) and hydrogenation of feedstock chemicals is very important in the context of ‘hydrogen storage’. Herein, we report a highly efficient reusable cobalt‐based heterogeneous catalyst for reversible dehydrogenation and hydrogenation of N‐heterocycles. Both the ADH and the hydrogenation processes operate under mild, benign conditions. Simple, efficient and mild: An efficient reusable cobalt‐based heterogeneous catalyst for reversible dehydrogenation and hydrogenation of N‐heterocycles is reported. Both processes are catalyzed by a single reusable cobalt‐catalyst that operates under mild and benign conditions.
ISSN:1867-3880
1867-3899
DOI:10.1002/cctc.201900367