Strong gate-tunability of flat bands in bilayer graphene due to moiré encapsulation between hBN monolayers

When using hexagonal boron-nitride (hBN) as a substrate for graphene, the resulting moiré pattern creates secondary Dirac points. By encapsulating a multilayer graphene within aligned hBN sheets the controlled moiré stacking may offer even richer benefits. Using advanced tight-binding simulations on...

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Published inNanoscale Vol. 15; no. 9; pp. 4561 - 4569
Main Authors Smeyers, Robin, Milošević, Milorad V, Covaci, Lucian
Format Journal Article
LanguageEnglish
Published England Royal Society of Chemistry 02.03.2023
Subjects
Bilayers
Encapsulation
Graphene
Heterostructures
Moire patterns
Multilayers
Stacking
Substrates
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Summary:When using hexagonal boron-nitride (hBN) as a substrate for graphene, the resulting moiré pattern creates secondary Dirac points. By encapsulating a multilayer graphene within aligned hBN sheets the controlled moiré stacking may offer even richer benefits. Using advanced tight-binding simulations on atomistically-relaxed heterostructures, here we show that the gap at the secondary Dirac point can be opened in selected moiré-stacking configurations, and is independent of any additional vertical gating of the heterostructure. On the other hand, gating can broadly tune the gap at the principal Dirac point, and may thereby strongly compress the first moiré mini-band in width against the moiré-induced gap at the secondary Dirac point. We reveal that in hBN-encapsulated bilayer graphene this novel mechanism can lead to isolated bands flatter than 10 meV under moderate gating, hence presenting a convenient pathway towards electronically-controlled strongly-correlated states on demand.
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ISSN:2040-3364
2040-3372
DOI:10.1039/d2nr07171a