Predicting heat generation in a lithium-ion pouch cell through thermography and the lumped capacitance model

• Published in: Journal of power sources Vol. 305; pp. 97 - 105
• Main Authors: Bazinski, S.J., Wang, X.
• Format: Journal Article
• Language: English
• Published: Elsevier B.V 15.02.2016
• Subjects: Lumped capacitance model; Thermography; Variable heat generation; Variable heat generation; Lumped capacitance model; Thermography
• ISSN: 0378-7753; 1873-2755
• DOI: 10.1016/j.jpowsour.2015.11.083

A technique is developed that combines a new closed-form analytical form of the lumped capacitance model (LCM) and thermography to predict the internal heat generation of a lithium-ion pouch cell. A series of tests is conducted to validate the new technique using a polyimide film heater mounted as a vertical plate in front of an infrared camera. A programmable power supply is used to subject the heater to three types of pre-defined heat profiles. The technique performs very well in reconstructing each known heat profile. The technique is then used to predict the rate of heat generation of a 14.5 Ah lithium iron phosphate cell under different rates of discharge. Compared to the heat rate measured by a calorimeter, the model predicts an average heat rate within 10% for moderate C-rates and lower. For C-rates higher than 2C, a simple correction algorithm is applied due to cell temperature gradients becoming more pronounced. •A closed-form lumped capacitance model is developed with varied heat generation.•Heat generation in a Lithium pouch cell is predicted from its surface temperature.•The new technique is validated using a 14.5 Ah Lithium iron phosphate pouch cell.