Surface plasmon effect combined with S-scheme charge migration in flower-like Ag/Ag6Si2O7/Bi12O17Cl2 enables efficient photocatalytic antibiotic degradation

A flower-like Ag/Ag6Si2O7/Bi12O17Cl2 plasmonic S-scheme heterojunction with is synthesized via a simple route. Under the synergistic cooperation of S-scheme heterostructure, and plasmonic effect, Ag/Ag6Si2O7/Bi12O17Cl2 exhibits exceptional photocatalytic properties toward antibiotic destruction unde...

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Published inApplied surface science Vol. 679; p. 161303
Main Authors Shen, Chuqi, Li, Xinyu, Xue, Bing, Feng, Diejing, Liu, Yanping, Yang, Fang, Zhang, Mingyi, Li, Shijie
Format Journal Article
LanguageEnglish
Published Elsevier B.V 15.01.2025
Subjects
Ag/Ag6Si2O7/Bi12O17Cl2
Antibiotic
Photocatalysis
Plasmonic effect
S-scheme heterojunction
Plasmonic effect
Antibiotic
Ag/Ag6Si2O7/Bi12O17Cl2
Photocatalysis
S-scheme heterojunction
Online AccessGet full text
ISSN0169-4332
DOI10.1016/j.apsusc.2024.161303

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Abstract A flower-like Ag/Ag6Si2O7/Bi12O17Cl2 plasmonic S-scheme heterojunction with is synthesized via a simple route. Under the synergistic cooperation of S-scheme heterostructure, and plasmonic effect, Ag/Ag6Si2O7/Bi12O17Cl2 exhibits exceptional photocatalytic properties toward antibiotic destruction under visible light irradiation. [Display omitted] •A plasmonic S-scheme heterojunction of Ag/Ag6Si2O7/Bi12O17Cl2 was synthesized.•Ag/Ag6Si2O7/Bi12O17Cl2 manifests superb photo-activity for antibiotic removal.•The photocatalytic mechanism, antibiotic degradation process and toxicities are analyzed.•The combination of S-scheme junction and plasmonic effect accounts for the reinforced catalytic performance. Developing robust photocatalysts for photocatalytic environment decontamination is significant and challenging. A novel flower-like S-scheme Ag/Ag6Si2O7/Bi12O17Cl2 (AASO/BOC) plasmonic heterojunction is successfully constructed using a facile route, and applied in photocatalytic destruction of tetracycline hydrochloride (TC) and levofloxacin (LEV) under visible-light irradiation. Benefiting from the combination of S-scheme Bi12O17Cl2/Ag6Si2O7 heterojunction and the plasma Ag, the production and separation of photogenerated carriers are dramatically enhanced. Consequently, compared to the pristine Bi12O17Cl2 and Ag6Si2O7, AASO/BOC displays superior photocatalytic degradation performance. Impressively, the photocatalytic TC degradation rate of AASO/BOC-2 reaches 0.0260 min−1, which is approximately 3.1, 14.4 and 2.0 times those of Bi12O17Cl2, Ag6Si2O7 and Bi12O17Cl2/Ag6Si2O7, respectively. Moreover, the photocatalytic mechanism of TC degradation is studied in depth via various techniques, and the photogenerated OH, O2− and h+ collectively contribute to the photo-degradation of TC. This research puts forward a neoteric approach to designing plasmonic S-scheme photocatalysts for environmental applications.
AbstractList A flower-like Ag/Ag6Si2O7/Bi12O17Cl2 plasmonic S-scheme heterojunction with is synthesized via a simple route. Under the synergistic cooperation of S-scheme heterostructure, and plasmonic effect, Ag/Ag6Si2O7/Bi12O17Cl2 exhibits exceptional photocatalytic properties toward antibiotic destruction under visible light irradiation. [Display omitted] •A plasmonic S-scheme heterojunction of Ag/Ag6Si2O7/Bi12O17Cl2 was synthesized.•Ag/Ag6Si2O7/Bi12O17Cl2 manifests superb photo-activity for antibiotic removal.•The photocatalytic mechanism, antibiotic degradation process and toxicities are analyzed.•The combination of S-scheme junction and plasmonic effect accounts for the reinforced catalytic performance. Developing robust photocatalysts for photocatalytic environment decontamination is significant and challenging. A novel flower-like S-scheme Ag/Ag6Si2O7/Bi12O17Cl2 (AASO/BOC) plasmonic heterojunction is successfully constructed using a facile route, and applied in photocatalytic destruction of tetracycline hydrochloride (TC) and levofloxacin (LEV) under visible-light irradiation. Benefiting from the combination of S-scheme Bi12O17Cl2/Ag6Si2O7 heterojunction and the plasma Ag, the production and separation of photogenerated carriers are dramatically enhanced. Consequently, compared to the pristine Bi12O17Cl2 and Ag6Si2O7, AASO/BOC displays superior photocatalytic degradation performance. Impressively, the photocatalytic TC degradation rate of AASO/BOC-2 reaches 0.0260 min−1, which is approximately 3.1, 14.4 and 2.0 times those of Bi12O17Cl2, Ag6Si2O7 and Bi12O17Cl2/Ag6Si2O7, respectively. Moreover, the photocatalytic mechanism of TC degradation is studied in depth via various techniques, and the photogenerated OH, O2− and h+ collectively contribute to the photo-degradation of TC. This research puts forward a neoteric approach to designing plasmonic S-scheme photocatalysts for environmental applications.
ArticleNumber 161303
Author Xue, Bing
Zhang, Mingyi
Li, Shijie
Feng, Diejing
Li, Xinyu
Liu, Yanping
Yang, Fang
Shen, Chuqi
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  surname: Shen
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  organization: Key Laboratory of Health Risk Factors for Seafood of Zhejiang Province, National Engineering Research Center for Marine Aquaculture, Zhejiang Ocean University, Zhoushan, Zhejiang Province 316022, China
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  givenname: Xinyu
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  organization: Key Laboratory of Health Risk Factors for Seafood of Zhejiang Province, National Engineering Research Center for Marine Aquaculture, Zhejiang Ocean University, Zhoushan, Zhejiang Province 316022, China
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  givenname: Bing
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  fullname: Xue, Bing
  organization: Key Laboratory of Health Risk Factors for Seafood of Zhejiang Province, National Engineering Research Center for Marine Aquaculture, Zhejiang Ocean University, Zhoushan, Zhejiang Province 316022, China
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  givenname: Diejing
  surname: Feng
  fullname: Feng, Diejing
  email: feng-dj@zjou.edu.cn
  organization: Key Laboratory of Health Risk Factors for Seafood of Zhejiang Province, National Engineering Research Center for Marine Aquaculture, Zhejiang Ocean University, Zhoushan, Zhejiang Province 316022, China
– sequence: 5
  givenname: Yanping
  surname: Liu
  fullname: Liu, Yanping
  organization: Key Laboratory of Health Risk Factors for Seafood of Zhejiang Province, National Engineering Research Center for Marine Aquaculture, Zhejiang Ocean University, Zhoushan, Zhejiang Province 316022, China
– sequence: 6
  givenname: Fang
  surname: Yang
  fullname: Yang, Fang
  organization: School of Mechanical and Automotive Engineering, Shanghai University of Engineering Science, Shanghai 201620, China
– sequence: 7
  givenname: Mingyi
  surname: Zhang
  fullname: Zhang, Mingyi
  email: zhangmingyi@hrbnu.edu.cn
  organization: Key Laboratory for Photonic and Electronic Bandgap Materials, Ministry of Education, School of Physics and Electronic Engineering, Harbin Normal University, Harbin 150025, China
– sequence: 8
  givenname: Shijie
  orcidid: 0000-0003-4635-5264
  surname: Li
  fullname: Li, Shijie
  email: lishijie@zjou.edu.cn
  organization: Key Laboratory of Health Risk Factors for Seafood of Zhejiang Province, National Engineering Research Center for Marine Aquaculture, Zhejiang Ocean University, Zhoushan, Zhejiang Province 316022, China
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Keywords Plasmonic effect
Antibiotic
Ag/Ag6Si2O7/Bi12O17Cl2
Photocatalysis
S-scheme heterojunction
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Snippet A flower-like Ag/Ag6Si2O7/Bi12O17Cl2 plasmonic S-scheme heterojunction with is synthesized via a simple route. Under the synergistic cooperation of S-scheme...
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StartPage 161303
SubjectTerms Ag/Ag6Si2O7/Bi12O17Cl2
Antibiotic
Photocatalysis
Plasmonic effect
S-scheme heterojunction
Title Surface plasmon effect combined with S-scheme charge migration in flower-like Ag/Ag6Si2O7/Bi12O17Cl2 enables efficient photocatalytic antibiotic degradation
URI https://dx.doi.org/10.1016/j.apsusc.2024.161303
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