Nucleation, aggregation, annealing, and disintegration of granular clusters

• Published in: Physical review. E, Statistical, nonlinear, and soft matter physics Vol. 89; no. 5; p. 052205
• Main Authors: González-Gutiérrez, Jorge, Carrillo-Estrada, J L, Ruiz-Suárez, J C
• Format: Journal Article
• Language: English
• Published: United States 01.05.2014
• Subjects: Colloids - chemistry; Computer Simulation; Crystallization - methods; Friction; Hardness; Magnetic Fields; Models, Chemical; Rheology - methods; Shear Strength; Stress, Mechanical; Vibration
• ISSN: 1550-2376
• DOI: 10.1103/PhysRevE.89.052205

The processes of nucleation, aggregation, annealing, and disintegration of clusters of non-Brownian paramagnetic beads in a vibrofluidized system are experimentally investigated. The interaction among the beads is induced by a magnetic seed composed of two dipoles allocated outside the container cell. We observe a clearly differentiated nucleation stage, whose evolution (nucleation time versus acceleration strength) follows a power law. Thereafter, the beads aggregate forming 2D disordered clusters around the nucleus. Both processes (nucleation and aggregation) are determined by the competition between magnetic forces and the drag produced by a thermal bath created by glass particles. Once the agglomerates reach a final state (shape and length), they are annealed by increasing and decreasing the granular temperature. We found that the fractal dimension and the lacunarity index clearly describe the structural variations of the clusters. Our discussion on this phenomenon is addressed, making a rough analogy with the glass transition in a super-cooled liquid. Finally, we study the disintegration of the clusters as a function of time and the density of the surrounding gas. The question is not if, but how they disintegrate upon removing the external field; we find that the disintegration follows an exponential decay.