MoS2 hydrogen evolution catalysis on p-Si nanorod photocathodes
We report on the synthesis of few−layers MoS2 flakes coated on the p−Si nanorods (p−SiNRs) via the metalorganic chemical vapor deposition (MOCVD) method. The MoS2 flakes show a vertically−standing, few−layers (10–15) morphology. The photoluminescence characteristic of the MoS2/p−SiNRs heterojunction...
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| Published in | Materials science in semiconductor processing Vol. 121; p. 105308 |
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| Main Authors | , , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
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Elsevier Ltd
01.01.2021
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| Abstract | We report on the synthesis of few−layers MoS2 flakes coated on the p−Si nanorods (p−SiNRs) via the metalorganic chemical vapor deposition (MOCVD) method. The MoS2 flakes show a vertically−standing, few−layers (10–15) morphology. The photoluminescence characteristic of the MoS2/p−SiNRs heterojunction exhibits a blue−shift energy bandgap (1.65−1.78 eV) at temperature of 77 K with thinner MoS2 layers due to the quantum confinement effect. As a result, the fabricated MoS2/p−SiNRs photocathode results in a saturated photocurrent density (PCD) and a photoconversion efficiency (η) of 42.3 mA cm−2, and 0.64% at 0 V (vs. RHE), respectively. Due to the built−in potential of heterojunction and more active edge sites, the onset voltage of the MoS2/p−SiNRs sample was positively shifted to ~0.72 V (vs. RHE). Based on this finding, we suggest that a heterojunction structure might serve an approach for fabricating the hybrid photoelectrochemical (PEC) device of the Si−based material.
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•Vertical-standing few-layer MoS2/p- Si nanorods were synthesized by the chemical etching, and CVD methods.•Photocurrent density and photoconversion efficiency of MoS2/p-Si nanorod-based photoelectrochemical cell (PEC) obtains 42.3 mA.cm-2, and 0.64%, respectively•The PEC device exhibits a positive onset potential of 0.72 V (vs. RHE) and the saturation current density is close to the JSC of the ideal solar cell. |
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| AbstractList | We report on the synthesis of few−layers MoS2 flakes coated on the p−Si nanorods (p−SiNRs) via the metalorganic chemical vapor deposition (MOCVD) method. The MoS2 flakes show a vertically−standing, few−layers (10–15) morphology. The photoluminescence characteristic of the MoS2/p−SiNRs heterojunction exhibits a blue−shift energy bandgap (1.65−1.78 eV) at temperature of 77 K with thinner MoS2 layers due to the quantum confinement effect. As a result, the fabricated MoS2/p−SiNRs photocathode results in a saturated photocurrent density (PCD) and a photoconversion efficiency (η) of 42.3 mA cm−2, and 0.64% at 0 V (vs. RHE), respectively. Due to the built−in potential of heterojunction and more active edge sites, the onset voltage of the MoS2/p−SiNRs sample was positively shifted to ~0.72 V (vs. RHE). Based on this finding, we suggest that a heterojunction structure might serve an approach for fabricating the hybrid photoelectrochemical (PEC) device of the Si−based material.
[Display omitted]
•Vertical-standing few-layer MoS2/p- Si nanorods were synthesized by the chemical etching, and CVD methods.•Photocurrent density and photoconversion efficiency of MoS2/p-Si nanorod-based photoelectrochemical cell (PEC) obtains 42.3 mA.cm-2, and 0.64%, respectively•The PEC device exhibits a positive onset potential of 0.72 V (vs. RHE) and the saturation current density is close to the JSC of the ideal solar cell. |
| ArticleNumber | 105308 |
| Author | Seo, Dong-Bum Tran, Thi Kim Chi Dang, Tran Chien Nguyen, Tien Dai Truong, Phuong Dung Nguyen, Viet Chien Man, Minh Tan Bui, Thi Thu Hien Dang, Van Thai Truong, Thi Hien Tran, Dai Lam Nguyen, Cao Khang Kim, Eui-Tae |
| Author_xml | – sequence: 1 givenname: Tran Chien surname: Dang fullname: Dang, Tran Chien organization: Institute of Theoretical and Applied Research, Duy Tan University, Hanoi, 100000, Vietnam – sequence: 2 givenname: Van Thai orcidid: 0000-0001-7916-6457 surname: Dang fullname: Dang, Van Thai organization: Institute of Theoretical and Applied Research, Duy Tan University, Hanoi, 100000, Vietnam – sequence: 3 givenname: Tien Dai surname: Nguyen fullname: Nguyen, Tien Dai email: nguyentiendai@duytan.edu.vn organization: Institute of Theoretical and Applied Research, Duy Tan University, Hanoi, 100000, Vietnam – sequence: 4 givenname: Thi Hien surname: Truong fullname: Truong, Thi Hien organization: Institute of Theoretical and Applied Research, Duy Tan University, Hanoi, 100000, Vietnam – sequence: 5 givenname: Minh Tan surname: Man fullname: Man, Minh Tan organization: Institute of Theoretical and Applied Research, Duy Tan University, Hanoi, 100000, Vietnam – sequence: 6 givenname: Thi Thu Hien surname: Bui fullname: Bui, Thi Thu Hien email: hienbtt@ims.vast.ac.vn organization: Institute of Materials Science, Vietnam Academy of Science and Technology, 18 Hoang Quoc Viet, Cau Giay, Hanoi, Vietnam – sequence: 7 givenname: Thi Kim Chi surname: Tran fullname: Tran, Thi Kim Chi organization: Graduate University of Science and Technology, Vietnam Academy of Science and Technology, 18 Hoang Quoc Viet, Cau Giay, Hanoi, Vietnam – sequence: 8 givenname: Dai Lam surname: Tran fullname: Tran, Dai Lam organization: Graduate University of Science and Technology, Vietnam Academy of Science and Technology, 18 Hoang Quoc Viet, Cau Giay, Hanoi, Vietnam – sequence: 9 givenname: Phuong Dung surname: Truong fullname: Truong, Phuong Dung organization: Institute of Geography, Vietnam Academy of Science and Technology, 18 Hoang Quoc Viet, Cau Giay, Hanoi, Vietnam – sequence: 10 givenname: Cao Khang surname: Nguyen fullname: Nguyen, Cao Khang organization: Center for Nano Science and Technology, Hanoi National University of Education, 136 Xuan Thuy, Cau Giay, Hanoi, Vietnam – sequence: 11 givenname: Viet Chien surname: Nguyen fullname: Nguyen, Viet Chien organization: University of Science & Technology, Daejeon, 34113, South Korea – sequence: 12 givenname: Dong-Bum surname: Seo fullname: Seo, Dong-Bum organization: Department of Materials Science & Engineering, Chungnam National University, Daejeon, 34134, South Korea – sequence: 13 givenname: Eui-Tae surname: Kim fullname: Kim, Eui-Tae organization: Department of Materials Science & Engineering, Chungnam National University, Daejeon, 34134, South Korea |
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| Title | MoS2 hydrogen evolution catalysis on p-Si nanorod photocathodes |
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