Halide-free deep eutectic solvents constructed from natural compounds for converting carbon dioxide to cyclic carbonate
Halide-free deep eutectic solvents (DESs) derived from natural biological compounds were used to gently catalyze the cycloaddition reaction between CO 2 and epoxides, with a TOF of 645 h −1 . The DFT calculation result was in good agreement with the experiment result, indicating that the ring closur...
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| Published in | Chemical communications (Cambridge, England) Vol. 61; no. 16; pp. 3391 - 3394 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
CAMBRIDGE
Royal Soc Chemistry
18.02.2025
Royal Society of Chemistry |
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| Abstract | Halide-free deep eutectic solvents (DESs) derived from natural biological compounds were used to gently catalyze the cycloaddition reaction between CO
2
and epoxides, with a TOF of 645 h
−1
. The DFT calculation result was in good agreement with the experiment result, indicating that the ring closure process was the rate-determining step.
Halide-free deep eutectic solvents (DESs) constructed from natural compounds were used to efficiently transform CO
2
into cyclic carbonates. |
|---|---|
| AbstractList | Halide-free deep eutectic solvents (DESs) derived from natural biological compounds were used to gently catalyze the cycloaddition reaction between CO
2
and epoxides, with a TOF of 645 h
−1
. The DFT calculation result was in good agreement with the experiment result, indicating that the ring closure process was the rate-determining step.
Halide-free deep eutectic solvents (DESs) constructed from natural compounds were used to efficiently transform CO
2
into cyclic carbonates. Halide-free deep eutectic solvents (DESs) derived from natural biological compounds were used to gently catalyze the cycloaddition reaction between CO 2 and epoxides, with a TOF of 645 h −1 . The DFT calculation result was in good agreement with the experiment result, indicating that the ring closure process was the rate-determining step. Halide-free deep eutectic solvents (DESs) derived from natural biological compounds were used to gently catalyze the cycloaddition reaction between CO and epoxides, with a TOF of 645 h . The DFT calculation result was in good agreement with the experiment result, indicating that the ring closure process was the rate-determining step. Halide-free deep eutectic solvents (DESs) derived from natural biological compounds were used to gently catalyze the cycloaddition reaction between CO2 and epoxides, with a TOF of 645 h-1. The DFT calculation result was in good agreement with the experiment result, indicating that the ring closure process was the rate-determining step.Halide-free deep eutectic solvents (DESs) derived from natural biological compounds were used to gently catalyze the cycloaddition reaction between CO2 and epoxides, with a TOF of 645 h-1. The DFT calculation result was in good agreement with the experiment result, indicating that the ring closure process was the rate-determining step. Halide-free deep eutectic solvents (DESs) derived from natural biological compounds were used to gently catalyze the cycloaddition reaction between CO2 and epoxides, with a TOF of 645 h−1. The DFT calculation result was in good agreement with the experiment result, indicating that the ring closure process was the rate-determining step. Halide-free deep eutectic solvents (DESs) derived from natural biological compounds were used to gently catalyze the cycloaddition reaction between CO2 and epoxides, with a TOF of 645 h-1. The DFT calculation result was in good agreement with the experiment result, indicating that the ring closure process was the rate-determining step. |
| Author | Chu, Dan-Dan Zhou, Jie Yu, Wen-Wang Meng, Xiang-Guang Li, Wen Ma, Xian-Jian |
| AuthorAffiliation | College of Chemistry Key Laboratory of Green Chemistry and Technology Ministry of Education Sichuan University |
| AuthorAffiliation_xml | – name: Sichuan University – name: College of Chemistry – name: Key Laboratory of Green Chemistry and Technology Ministry of Education |
| Author_xml | – sequence: 1 givenname: Wen-Wang surname: Yu fullname: Yu, Wen-Wang – sequence: 2 givenname: Xiang-Guang surname: Meng fullname: Meng, Xiang-Guang – sequence: 3 givenname: Wen surname: Li fullname: Li, Wen – sequence: 4 givenname: Jie surname: Zhou fullname: Zhou, Jie – sequence: 5 givenname: Xian-Jian surname: Ma fullname: Ma, Xian-Jian – sequence: 6 givenname: Dan-Dan surname: Chu fullname: Chu, Dan-Dan |
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| Cites_doi | 10.1038/s41467-019-13638-9 10.1021/acs.chemrev.0c00883 10.1039/d2gc02517e 10.1016/j.jcou.2020.101302 10.1007/s10311-022-01470-5 10.1039/d2gc02146c 10.1016/j.cej.2022.138715 10.3390/molecules27249006 10.1016/j.mcat.2023.113812 10.1039/c7ta08629f 10.1016/j.gee.2019.03.002 10.2174/0122133461255437230930182648 10.1021/sc500096j 10.1002/cctc.202201373 10.1039/c2cs35178a 10.1016/j.jcou.2023.102659 10.1016/j.cogsc.2020.04.002 10.1021/acs.inorgchem.3c01899 10.1021/acssuschemeng.2c03210 10.1039/D2GC02517E 10.1039/D2GC02146C 10.1039/C7TA08629F |
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| Snippet | Halide-free deep eutectic solvents (DESs) derived from natural biological compounds were used to gently catalyze the cycloaddition reaction between CO
2
and... Halide-free deep eutectic solvents (DESs) derived from natural biological compounds were used to gently catalyze the cycloaddition reaction between CO2 and... Halide-free deep eutectic solvents (DESs) derived from natural biological compounds were used to gently catalyze the cycloaddition reaction between CO 2 and... Halide-free deep eutectic solvents (DESs) derived from natural biological compounds were used to gently catalyze the cycloaddition reaction between CO and... |
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| SubjectTerms | Carbon dioxide Chemistry Chemistry, Multidisciplinary Cycloaddition Eutectic reactions Physical Sciences Science & Technology Solvents |
| Title | Halide-free deep eutectic solvents constructed from natural compounds for converting carbon dioxide to cyclic carbonate |
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