Evaluation of the mixing quality of high-viscosity yield stress fluids in a tubular reactor

• Published in: International journal of chemical reactor engineering Vol. 19; no. 6; pp. 625 - 635
• Main Authors: Xie, Le, He, Guangwen, Yu, Bin, Yan, Shaowei
• Format: Journal Article
• Language: English
• Published: De Gruyter 2021
• Subjects: computational fluid dynamics; large eddy simulation; mixing; non-Newtonian fluid
• ISSN: 2194-5748; 1542-6580
• DOI: 10.1515/ijcre-2020-0237

In this study, the mixing quality of high-viscosity yield stress fluid (Carbopol aqueous solution) under laminar and turbulent flow regimes was evaluated through a numerical experimental study. A three-dimensional computational fluid dynamics large-eddy simulation (CFD-LES) model was employed to capture large-scale vortex structures. The proposed CFD model was validated by the experimental data in terms of mean velocity profiles and velocity-time history. Thereafter, the CFD model was applied to simulate the residence time distribution using the tracking technique: tracer pulse method and step method. In addition, the non-ideal flow phenomena caused by molecular diffusion and eddy diffusion were evaluated. The effects of the rheological properties on the mixing performance were also investigated. The presented results can provide useful guidance to enhance mass transfer in reactors with high-viscosity fluids.