Alternative anodes for low temperature lithium-ion batteries
Li-ion batteries (LIBs) have become critical components in the manufacture of electric vehicles (EVs) as they offer the best all-round performance compared to competing battery chemistries. However, LIB performance at low temperature (LT) extremes of EV operation (typically −40 to 0 °C) suffers from...
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Published in | Journal of materials chemistry. A, Materials for energy and sustainability Vol. 9; no. 25; pp. 14172 - 14213 |
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Main Authors | , , |
Format | Journal Article |
Language | English |
Published |
Cambridge
Royal Society of Chemistry
07.07.2021
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Abstract | Li-ion batteries (LIBs) have become critical components in the manufacture of electric vehicles (EVs) as they offer the best all-round performance compared to competing battery chemistries. However, LIB performance at low temperature (LT) extremes of EV operation (typically −40 to 0 °C) suffers from a reduced output and diminished cycle life. LT cycling increases cell impedance, diminishing Li ion diffusion through the cell, exacerbating electrode polarisation, and hindering interfacial Li
+
desolvation. Herein, we present a comprehensive review of (i) the factors that influence LT Li-ion performance, (ii) outline the shortcomings of the current state-of-the-art and (iii) discuss recent findings in the field, focusing on alternative anode materials with particular emphasis on high-capacity, fast charging alternatives to the archetypal carbon (graphite) anode. Different approaches to improve LT LIB performance are outlined in an in-depth analysis of recent improvements from the anode perspective. These include electrolyte-driven enhancements, the resurgence of Li metal batteries, the impact of conductive coatings, elemental doping and nanocomposite formation, substitution of intercalating anodes with high-capacity Li alloying and Li conversion materials, and fast redox pseudocapacitance.
Major issues of commercial graphite-based Li-ion batteries at low temperature and recent improvements in anode formulation to tackle these low temperature limitations. |
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AbstractList | Li-ion batteries (LIBs) have become critical components in the manufacture of electric vehicles (EVs) as they offer the best all-round performance compared to competing battery chemistries. However, LIB performance at low temperature (LT) extremes of EV operation (typically −40 to 0 °C) suffers from a reduced output and diminished cycle life. LT cycling increases cell impedance, diminishing Li ion diffusion through the cell, exacerbating electrode polarisation, and hindering interfacial Li + desolvation. Herein, we present a comprehensive review of (i) the factors that influence LT Li-ion performance, (ii) outline the shortcomings of the current state-of-the-art and (iii) discuss recent findings in the field, focusing on alternative anode materials with particular emphasis on high-capacity, fast charging alternatives to the archetypal carbon (graphite) anode. Different approaches to improve LT LIB performance are outlined in an in-depth analysis of recent improvements from the anode perspective. These include electrolyte-driven enhancements, the resurgence of Li metal batteries, the impact of conductive coatings, elemental doping and nanocomposite formation, substitution of intercalating anodes with high-capacity Li alloying and Li conversion materials, and fast redox pseudocapacitance. Li-ion batteries (LIBs) have become critical components in the manufacture of electric vehicles (EVs) as they offer the best all-round performance compared to competing battery chemistries. However, LIB performance at low temperature (LT) extremes of EV operation (typically −40 to 0 °C) suffers from a reduced output and diminished cycle life. LT cycling increases cell impedance, diminishing Li ion diffusion through the cell, exacerbating electrode polarisation, and hindering interfacial Li + desolvation. Herein, we present a comprehensive review of (i) the factors that influence LT Li-ion performance, (ii) outline the shortcomings of the current state-of-the-art and (iii) discuss recent findings in the field, focusing on alternative anode materials with particular emphasis on high-capacity, fast charging alternatives to the archetypal carbon (graphite) anode. Different approaches to improve LT LIB performance are outlined in an in-depth analysis of recent improvements from the anode perspective. These include electrolyte-driven enhancements, the resurgence of Li metal batteries, the impact of conductive coatings, elemental doping and nanocomposite formation, substitution of intercalating anodes with high-capacity Li alloying and Li conversion materials, and fast redox pseudocapacitance. Major issues of commercial graphite-based Li-ion batteries at low temperature and recent improvements in anode formulation to tackle these low temperature limitations. |
Author | Collins, Gearoid A Ryan, Kevin M Geaney, Hugh |
AuthorAffiliation | University of Limerick Department of Chemical Sciences and Bernal Institute |
AuthorAffiliation_xml | – name: Department of Chemical Sciences and Bernal Institute – name: University of Limerick |
Author_xml | – sequence: 1 givenname: Gearoid A surname: Collins fullname: Collins, Gearoid A – sequence: 2 givenname: Hugh surname: Geaney fullname: Geaney, Hugh – sequence: 3 givenname: Kevin M surname: Ryan fullname: Ryan, Kevin M |
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Notes | which has 16 partners across Europe. He currently holds IRC laureate and SFI Investigator awards. He has a h-index of 40 with >130 publications with interests in nanomaterial synthesis and their application as alloying materials in rechargeable batteries. He is a Co-Principal Investigator on Science Foundation Ireland Research Centres, MaREI and AMBER and Funded Investigator in the centres Confirm and SSPC. He is coordinator of the Horizon 2020 project Si-Drive 2 Professor Kevin M. Ryan holds a Personal Chair in Chemical Nanotechnology at the Department of Chemical Sciences and Bernal Institute at the University of Limerick in Ireland http://geaneygroupul.ie/ www.ryangroupul.ie https://sidrive2020.eu/ batteries in University College Cork, before returning to the University of Limerick, where he was the recipient of a Starting Investigator Research Grant (SIRG) from Science Foundation Ireland. He is currently a lecturer in Chemistry in the Department of Chemical Sciences in the University of Limerick, and carries out research within the Bernal Institute. His research interests are in Li-ion and beyond Li-ion batteries (specifically Na-ion, Li-S and Al-ion). Details on his research focus and output can be found at Gearóid Collins received his undergraduate degree in Nanoscience from Trinity College, Dublin in 2017. He is currently a final year PhD candidate at the University of Limerick, in partnership with the Irish Research Council and Intel Ireland. He is researching bottom-up growth of nanostructured anode materials for energy-dense lithium-ion batteries. His areas of research focus on developing highly conductive nanowire (NW)-based anodes for low temperature applications; overcoming loading limitations of directly-grown Si NWs through the use of nanotextured 3D growth templates; scalable synthesis of Si NW/graphite composites; and investigating the utility of nanostructured conversion materials as suitable battery anodes. Dr Hugh Geaney received his BSc. in Industrial Chemistry and PhD from the University of Limerick, Ireland. He carried out postdoctoral research on Li-O . |
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ParticipantIDs | proquest_journals_2545974545 crossref_primary_10_1039_D1TA00998B rsc_primary_d1ta00998b |
PublicationCentury | 2000 |
PublicationDate | 2021-07-07 |
PublicationDateYYYYMMDD | 2021-07-07 |
PublicationDate_xml | – month: 07 year: 2021 text: 2021-07-07 day: 07 |
PublicationDecade | 2020 |
PublicationPlace | Cambridge |
PublicationPlace_xml | – name: Cambridge |
PublicationTitle | Journal of materials chemistry. A, Materials for energy and sustainability |
PublicationYear | 2021 |
Publisher | Royal Society of Chemistry |
Publisher_xml | – name: Royal Society of Chemistry |
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SubjectTerms | Anodes Batteries Critical components Electric vehicles Electrode materials Electrode polarization Ion diffusion Lithium Lithium-ion batteries Low temperature Nanocomposites Rechargeable batteries |
Title | Alternative anodes for low temperature lithium-ion batteries |
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