BaF radical: A promising candidate for laser cooling and magneto-optical trapping

Recently, there have been great interest and advancement in the field of laser cooling and magneto-optical trapping of molecules. The rich internal structure of molecules naturally lends themselves to extensive and exciting applications. In this paper, the radical 138Ba19F, as a promising candidate...

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Bibliographic Details
Published inChinese physics B Vol. 26; no. 3; pp. 321 - 329
Main Author 许亮 魏斌 夏勇 邓联忠 印建平
Format Journal Article
LanguageEnglish
Published 01.03.2017
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ISSN1674-1056
2058-3834
DOI10.1088/1674-1056/26/3/033702

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Summary:Recently, there have been great interest and advancement in the field of laser cooling and magneto-optical trapping of molecules. The rich internal structure of molecules naturally lends themselves to extensive and exciting applications. In this paper, the radical 138Ba19F, as a promising candidate for laser cooling and magneto-optical trapping, is discussed in detail.The highly diagonal Franck-Condon factors between theX2∑+1/2and A2∏1/2states are first confirmed with three different methods. Afterwards, with the effective Hamiltonian approach and irreducible tensor theory, the hypertine structure of theX2∑+1/2state is calculated accurately. A scheme for laser cooling is given clearly. Besides, the Zeeman effects of the upper ( A2∏1/2)andlower(X2∑+1/2)levels are also studied, and their respective g factors are obtained under a weak magnetic field. Its large g factor of the upper stateA2∏1/2is advantageous for magneto-optical trapping. Finally, by studying Stark effect of BaFin theX2∑+1/2, we investigate the dependence of the internal effective electric field on the applied electric field. It is suggested that such a laser-cooled BaF is also a promising candidate for precision measurement of electron electric dipole moment.
Bibliography:Liang Xu, Bin Wei, Yong Xia, Lian-Zhong Deng, and Jian-Ping Yin(State Key Laboratory of Precision Spectroscopy, School of Physics and Materials Science, East China Normal University, Shanghai 200062, China)
laser cooling, magneto-optical trapping, BaF radical
11-5639/O4
Recently, there have been great interest and advancement in the field of laser cooling and magneto-optical trapping of molecules. The rich internal structure of molecules naturally lends themselves to extensive and exciting applications. In this paper, the radical 138Ba19F, as a promising candidate for laser cooling and magneto-optical trapping, is discussed in detail.The highly diagonal Franck-Condon factors between theX2∑+1/2and A2∏1/2states are first confirmed with three different methods. Afterwards, with the effective Hamiltonian approach and irreducible tensor theory, the hypertine structure of theX2∑+1/2state is calculated accurately. A scheme for laser cooling is given clearly. Besides, the Zeeman effects of the upper ( A2∏1/2)andlower(X2∑+1/2)levels are also studied, and their respective g factors are obtained under a weak magnetic field. Its large g factor of the upper stateA2∏1/2is advantageous for magneto-optical trapping. Finally, by studying Stark effect of BaFin theX2∑+1/2, we investigate the dependence of the internal effective electric field on the applied electric field. It is suggested that such a laser-cooled BaF is also a promising candidate for precision measurement of electron electric dipole moment.
ISSN:1674-1056
2058-3834
DOI:10.1088/1674-1056/26/3/033702