Emulsions in microfluidic channels with asymmetric boundary conditions and directional surface roughness: stress and rheology

• Published in: Soft matter Vol. 2; no. 26; pp. 523 - 5211
• Main Authors: Pelusi, Francesca, Filippi, Daniele, Derzsi, Ladislav, Pierno, Matteo, Sbragaglia, Mauro
• Format: Journal Article
• Language: English
• Published: England Royal Society of Chemistry 03.07.2024
• Subjects: Asymmetry; Boundary conditions; Channels; Emulsions; Microfluidics; Rheological properties; Rheology; Surface roughness; Velocity; Velocity distribution
• ISSN: 1744-683X; 1744-6848; 1744-6848
• DOI: 10.1039/d4sm00041b

The flow of emulsions in confined microfluidic channels is affected by surface roughness. Directional roughness effects have recently been reported in channels with asymmetric boundary conditions featuring a flat wall, and a wall textured with directional roughness, the latter promoting a change in the velocity profiles when the flow direction of emulsions is inverted [D. Filippi et al. , Adv. Mater. Technol. , 2023, 8 , 2201748]. An operative protocol is needed to reconstruct the stress profile inside the channel from velocity data to shed light on the trigger of the directional response. To this aim, we performed lattice Boltzmann numerical simulations of the flow of model emulsions with a minimalist model of directional roughness in two dimensions: a confined microfluidic channel with one flat wall and the other patterned by right-angle triangular-shaped posts. Simulations are essential to develop a protocol based on mechanical arguments to reconstruct stress profiles. Hence, one can analyze data to relate directional effects in velocity profiles to different rheological responses close to the rough walls associated with opposite flow directions. We finally show the universality of this protocol by applying it to other realizations of directional roughness by considering experimental data on emulsions in a microfluidic channel featuring a flat wall and a wall textured by herringbone-shaped roughness. Numerical simulations help in elaborating a validated protocol for reconstructing stress profiles in channels with asymmetric boundary conditions and directional roughness, which is crucial for investigating rheological responses near the rough wall.