Acetic acid formation from methane and carbon dioxide via non-thermal plasma reactions towards an effective carbon fixation

While direct CH 3 COOH formation from CH 4 and CO 2 in a non-equilibrium condition is an ideal process, a dielectric-barrier discharge plasma reaction in the presence of CO 2 and isotopic CH 4 ( 13 CH 4 ) revealed that the primly produced CH 3 COOH can comprise both CH 4 -derived carbons ( i.e. , no...

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Bibliographic Details
Published inNew journal of chemistry Vol. 46; no. 17; pp. 7855 - 7858
Main Authors Nishimura, Naoyuki, Akaogi, Takayuki, Onishi, Kazuhiro, Tojo, Masahiro
Format Journal Article
LanguageEnglish
Published Cambridge Royal Society of Chemistry 03.05.2022
Subjects
Acetic acid
Carbon dioxide
Dielectric barrier discharge
Equilibrium conditions
Fixation
Methane
Thermal plasmas
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Summary:While direct CH 3 COOH formation from CH 4 and CO 2 in a non-equilibrium condition is an ideal process, a dielectric-barrier discharge plasma reaction in the presence of CO 2 and isotopic CH 4 ( 13 CH 4 ) revealed that the primly produced CH 3 COOH can comprise both CH 4 -derived carbons ( i.e. , no CO 2 -derived carbon), indicating the importance of a particular CO 2 activation control in non-thermal plasma for an effective carbon fixation.
ISSN:1144-0546
1369-9261
DOI:10.1039/D2NJ00409G