A new approach to ignition time prediction in crude oil oxidation using PDSC
•In-situ combustion ignition time was estimated with a new approach based on PDSC.•Time estimation depends on heat release time exponential dependence on φ-factor.•Oil A and B showed an oxidation delay of 27 days and 8.8 months, respectively.•Our results were applied in two pilot projects for 2 crud...
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| Published in | Fuel (Guildford) Vol. 353; p. 128940 |
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| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
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Elsevier Ltd
01.12.2023
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| Abstract | •In-situ combustion ignition time was estimated with a new approach based on PDSC.•Time estimation depends on heat release time exponential dependence on φ-factor.•Oil A and B showed an oxidation delay of 27 days and 8.8 months, respectively.•Our results were applied in two pilot projects for 2 crude oils field.•Oil A showed self-ignition meanwhile oil B required artificial ignition.
In-situ combustion process is recognized as being one of the promising methods in the field of enhanced oil recovery. In this study, we developed a procedure for estimating ignition time using pressurized differential scanning calorimetric technique (PDSC) and the chain reaction ignition approach. The procedure was based on the free-radical mechanism of oxidation and was successfully applied to PDSC kinetic curves processing. The initial stages of oxidation of crude oils A and B were studied in detail. It was found that the procedure for processing the oils' activity to oxidation was characterized by a heat release time exponential dependence factor (φ − factor). Even though oil A and oil B exhibit comparable kinetic parameters of oxidation, there is a marked difference in their behavior. Oil A demonstrated an induction period of 27 days and a φ value of 0.0123. Conversely, oil B did not initiate combustion within a suitable timeframe in-situ, and presented a lower φ value of 0.0067. The results of pilot tests using oil A and B were consistent with the predictions and demonstrated the potential of the proposed approach. |
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| AbstractList | •In-situ combustion ignition time was estimated with a new approach based on PDSC.•Time estimation depends on heat release time exponential dependence on φ-factor.•Oil A and B showed an oxidation delay of 27 days and 8.8 months, respectively.•Our results were applied in two pilot projects for 2 crude oils field.•Oil A showed self-ignition meanwhile oil B required artificial ignition.
In-situ combustion process is recognized as being one of the promising methods in the field of enhanced oil recovery. In this study, we developed a procedure for estimating ignition time using pressurized differential scanning calorimetric technique (PDSC) and the chain reaction ignition approach. The procedure was based on the free-radical mechanism of oxidation and was successfully applied to PDSC kinetic curves processing. The initial stages of oxidation of crude oils A and B were studied in detail. It was found that the procedure for processing the oils' activity to oxidation was characterized by a heat release time exponential dependence factor (φ − factor). Even though oil A and oil B exhibit comparable kinetic parameters of oxidation, there is a marked difference in their behavior. Oil A demonstrated an induction period of 27 days and a φ value of 0.0123. Conversely, oil B did not initiate combustion within a suitable timeframe in-situ, and presented a lower φ value of 0.0067. The results of pilot tests using oil A and B were consistent with the predictions and demonstrated the potential of the proposed approach. |
| ArticleNumber | 128940 |
| Author | Vakhin, Alexey V. Gilmanova, Rasima Kh Ushakova, Alexandra S. Khelkhal, Mohammed A. Zatsepin, Vladislav V. |
| Author_xml | – sequence: 1 givenname: Alexandra S. orcidid: 0000-0002-6717-7316 surname: Ushakova fullname: Ushakova, Alexandra S. organization: A. N. Nesmeyanov Institute of Organoelement Compounds RAS, Vavilova ul., 28, Moscow, Russia – sequence: 2 givenname: Vladislav V. surname: Zatsepin fullname: Zatsepin, Vladislav V. organization: Bashkir State University, st. aki Validi, 32, Ufa, Bashkortostan 450076, Russia – sequence: 3 givenname: Mohammed A. surname: Khelkhal fullname: Khelkhal, Mohammed A. email: MHelhal@kpfu.ru organization: Institute of Geology and Petroleum Technologies, Kazan Federal University, Kazan 420008, Russia – sequence: 4 givenname: Alexey V. surname: Vakhin fullname: Vakhin, Alexey V. organization: Institute of Geology and Petroleum Technologies, Kazan Federal University, Kazan 420008, Russia – sequence: 5 givenname: Rasima Kh surname: Gilmanova fullname: Gilmanova, Rasima Kh organization: LLC NPO “Neftegaztekhnologiya”, Revolutsionnaya str., 96/2, Ufa, Bashkortostan 450078, Russia |
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| Keywords | Air injection HPAI Chain reaction In-situ combustion Enhanced oil recovery PDC |
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| SubjectTerms | Air injection Chain reaction Enhanced oil recovery HPAI In-situ combustion PDC |
| Title | A new approach to ignition time prediction in crude oil oxidation using PDSC |
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