Assessing residential PM 2.5 concentrations and infiltration factors with high spatiotemporal resolution using crowdsourced sensors

• Published in: Proceedings of the National Academy of Sciences - PNAS Vol. 120; no. 50; p. e2308832120
• Main Authors: Lunderberg, David M, Liang, Yutong, Singer, Brett C, Apte, Joshua S, Nazaroff, William W, Goldstein, Allen H
• Format: Journal Article
• Language: English
• Published: United States 12.12.2023
• Subjects: Air Pollutants - analysis; Air Pollution, Indoor - analysis; Crowdsourcing; Environmental Monitoring; Humans; Particle Size; Particulate Matter - analysis; exposure; indoor air; source apportionment; infiltration; PM2.5
• ISSN: 0027-8424; 1091-6490
• DOI: 10.1073/pnas.2308832120

Building conditions, outdoor climate, and human behavior influence residential concentrations of fine particulate matter (PM ). To study PM spatiotemporal variability in residences, we acquired paired indoor and outdoor PM measurements at 3,977 residences across the United States totaling >10,000 monitor-years of time-resolved data (10-min resolution) from the PurpleAir network. Time-series analysis and statistical modeling apportioned residential PM concentrations to outdoor sources (median residential contribution = 52% of total, coefficient of variation = 69%), episodic indoor emission events such as cooking (28%, CV = 210%) and persistent indoor sources (20%, CV = 112%). Residences in the temperate marine climate zone experienced higher infiltration factors, consistent with expectations for more time with open windows in milder climates. Likewise, for all climate zones, infiltration factors were highest in summer and lowest in winter, decreasing by approximately half in most climate zones. Large outdoor-indoor temperature differences were associated with lower infiltration factors, suggesting particle losses from active filtration occurred during heating and cooling. Absolute contributions from both outdoor and indoor sources increased during wildfire events. Infiltration factors decreased during periods of high outdoor PM , such as during wildfires, reducing potential exposures from outdoor-origin particles but increasing potential exposures to indoor-origin particles. Time-of-day analysis reveals that episodic emission events are most frequent during mealtimes as well as on holidays (Thanksgiving and Christmas), indicating that cooking-related activities are a strong episodic emission source of indoor PM in monitored residences.