Energy-scaling of the product state distribution for three-body recombination of ultracold atoms

Three-body recombination is a chemical reaction where the collision of three atoms leads to the formation of a diatomic molecule. In the ultracold regime it is expected that the production rate of a molecule generally decreases with its binding energy \(E_b\), however, its precise dependence and the...

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Published inarXiv.org
Main Authors Haze, Shinsuke, D'Incao, José P, Dorer, Dominik, Li, Jinglun, Markus Dei\ss, Tiemann, Eberhard, Julienne, Paul S, Johannes Hecker Denschlag
Format Paper Journal Article
LanguageEnglish
Published Ithaca Cornell University Library, arXiv.org 09.11.2022
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Summary:Three-body recombination is a chemical reaction where the collision of three atoms leads to the formation of a diatomic molecule. In the ultracold regime it is expected that the production rate of a molecule generally decreases with its binding energy \(E_b\), however, its precise dependence and the physics governing it have been left unclear so far. Here, we present a comprehensive experimental and theoretical study of the energy dependency for three-body recombination of ultracold Rb. For this, we determine production rates for molecules in a state-to-state resolved manner, with the binding energies \(E_b\) ranging from 0.02 to 77 GHz\(\times h\). We find that the formation rate approximately scales as \(E_b^{-\alpha}\), where \(\alpha\) is in the vicinity of 1. The formation rate typically varies only within a factor of two for different rotational angular momenta of the molecular product, apart from a possible centrifugal barrier suppression for low binding energies. In addition to numerical three-body calculations we present a perturbative model which reveals the physical origin of the energy scaling of the formation rate. Furthermore, we show that the scaling law potentially holds universally for a broad range of interaction potentials.
ISSN:2331-8422
DOI:10.48550/arxiv.2211.03834