Confirmation of Kramers-Henneberger Atoms

In a remarkable experiment, Eichmann et al. attained unprecedented acceleration of neutral atoms by strong short-pulse IR laser fields. The driving mechanism was identified as the ponderomotive force on excited electrons bound in Rydberg orbits that survive long enough to enable the atoms to reach t...

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Bibliographic Details
Main Authors Wei, Qi, Wang, Pingxiao, Kais, Sabre, Herschbach, Dudley
Format Journal Article
LanguageEnglish
Published 06.09.2016
Subjects
Physics - Atomic Physics
Physics - Optics
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Summary:In a remarkable experiment, Eichmann et al. attained unprecedented acceleration of neutral atoms by strong short-pulse IR laser fields. The driving mechanism was identified as the ponderomotive force on excited electrons bound in Rydberg orbits that survive long enough to enable the atoms to reach the detector. However, the observed velocities lie somewhat above the theoretical prediction. The systematic discrepancy was attributed to "absolute laser intensity uncertainties or a slightly non-Gaussian intensity distribution". Here, we examine the process by transforming to the Kramers-Henneberger (KH) reference frame. We find that in addition to the ponderomotive potential there exists a smaller but significant term that comes from the binding energy of the KH atom. Including this KH term brings the calculated maximum velocities to a close match with experimental results over the full range of laser pulse durations.
DOI:10.48550/arxiv.1609.01434