Spatiotemporal chaos and quasipatterns in coupled reaction-diffusion systems

• Published in: arXiv.org
• Main Authors: Castelino, Jennifer K, Ratliff, Daniel J, Rucklidge, Alastair M, Subramanian, Priya, Topaz, Chad M
• Format: Paper Journal Article
• Language: English
• Published: Ithaca Cornell University Library, arXiv.org 20.03.2020
• Subjects: Computer simulation; Coupled modes; Mathematical models; Organic chemistry; Physics - Pattern Formation and Solitons; Wave interaction
• ISSN: 2331-8422
• DOI: 10.48550/arxiv.2001.11730

In coupled reaction-diffusion systems, modes with two different length scales can interact to produce a wide variety of spatiotemporal patterns. Three-wave interactions between these modes can explain the occurrence of spatially complex steady patterns and time-varying states including spatiotemporal chaos. The interactions can take the form of two short waves with different orientations interacting with one long wave, or vice-versa. We investigate the role of such three-wave interactions in a coupled Brusselator system. As well as finding simple steady patterns when the waves reinforce each other, we can also find spatially complex but steady patterns, including quasipatterns. When the waves compete with each other, time varying states such as spatiotemporal chaos are also possible. The signs of the quadratic coefficients in three-wave interaction equations distinguish between these two cases. By manipulating parameters of the chemical model, the formation of these various states can be encouraged, as we confirm through extensive numerical simulation. Our arguments allow us to predict when spatiotemporal chaos might be found: standard nonlinear methods fail in this case. The arguments are quite general and apply to a wide class of pattern-forming systems, including the Faraday wave experiment.