Radiative deflection of a BaF molecular beam from the optical cycling

We demonstrate a quasi optical cycling for the \(X(v=0)\to A(v'=0)\) transition and a radiative force induced deflection on the buffer-gas cooled BaF molecular beam. The laser induced fluorescence enhancement with additional sidebands and a polarization modulation scheme indicates that the hype...

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Bibliographic Details
Published inarXiv.org
Main Authors Chen, Tao, Bu, Wenhao, Yan, Bo
Format Paper Journal Article
LanguageEnglish
Published Ithaca Cornell University Library, arXiv.org 22.09.2017
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Summary:We demonstrate a quasi optical cycling for the \(X(v=0)\to A(v'=0)\) transition and a radiative force induced deflection on the buffer-gas cooled BaF molecular beam. The laser induced fluorescence enhancement with additional sidebands and a polarization modulation scheme indicates that the hyperfine states and the Zeeman sublevels are closed. The quasi optical cycling by repumping the \(X(v=1)\to A(v'=0)\) leads to a \(\sim\) 0.8 mm deflection of the beam via scattering \(\sim\) 150 photons per molecule, in good agreement with the predictions from our multi-level rate equation model. Further improvement by closing the leakage \(X(v=2)\) and \(\Delta\) state allows scattering thousands of photons, and laser cooling and slowing of BaF.
ISSN:2331-8422
DOI:10.48550/arxiv.1709.07602