Magnetoelectric effect and phase transitions in CuO in external magnetic fields
Apart from being so far the only known binary multiferroic compound, CuO has a much higher transition temperature into the multiferroic state, 230 K, than any other known material in which the electric polarization is induced by spontaneous magnetic order, typically lower than 100 K. Although the ma...
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Abstract | Apart from being so far the only known binary multiferroic compound, CuO has a much higher transition temperature into the multiferroic state, 230 K, than any other known material in which the electric polarization is induced by spontaneous magnetic order, typically lower than 100 K. Although the magnetically induced ferroelectricity of CuO is firmly established, no magnetoelectric effect has been observed so far as direct crosstalk between bulk magnetization and electric polarization counterparts. Here we demonstrate that high magnetic fields of about 50 T are able to suppress the helical modulation of the spins in the multiferroic phase and dramatically affect the electric polarization. Furthermore, just below the spontaneous transition from commensurate (paraelectric) to incommensurate (ferroelectric) structures at 213 K, even modest magnetic fields induce a transition into the incommensurate structure and then suppress it at higher field. Thus, remarkable hidden magnetoelectric features are uncovered, establishing CuO as prototype multiferroic with abundance of competitive magnetic interactions. |
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AbstractList | Nat. Commun. 7, 10295 (2016) Apart from being so far the only known binary multiferroic compound, CuO has
a much higher transition temperature into the multiferroic state, 230 K, than
any other known material in which the electric polarization is induced by
spontaneous magnetic order, typically lower than 100 K. Although the
magnetically induced ferroelectricity of CuO is firmly established, no
magnetoelectric effect has been observed so far as direct crosstalk between
bulk magnetization and electric polarization counterparts. Here we demonstrate
that high magnetic fields of about 50 T are able to suppress the helical
modulation of the spins in the multiferroic phase and dramatically affect the
electric polarization. Furthermore, just below the spontaneous transition from
commensurate (paraelectric) to incommensurate (ferroelectric) structures at 213
K, even modest magnetic fields induce a transition into the incommensurate
structure and then suppress it at higher field. Thus, remarkable hidden
magnetoelectric features are uncovered, establishing CuO as prototype
multiferroic with abundance of competitive magnetic interactions. Apart from being so far the only known binary multiferroic compound, CuO has a much higher transition temperature into the multiferroic state, 230 K, than any other known material in which the electric polarization is induced by spontaneous magnetic order, typically lower than 100 K. Although the magnetically induced ferroelectricity of CuO is firmly established, no magnetoelectric effect has been observed so far as direct crosstalk between bulk magnetization and electric polarization counterparts. Here we demonstrate that high magnetic fields of about 50 T are able to suppress the helical modulation of the spins in the multiferroic phase and dramatically affect the electric polarization. Furthermore, just below the spontaneous transition from commensurate (paraelectric) to incommensurate (ferroelectric) structures at 213 K, even modest magnetic fields induce a transition into the incommensurate structure and then suppress it at higher field. Thus, remarkable hidden magnetoelectric features are uncovered, establishing CuO as prototype multiferroic with abundance of competitive magnetic interactions. |
Author | Skumryev, Vassil Wang, Zhaosheng Yasin, Shadi Ivanov, Vsevolod Ressouche, Eric Skourski, Yurii Geshev, Julian Qureshi, Navid Zherlitsyn, Sergei Mukhin, Alexander Gospodinov, Marin |
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BackLink | https://doi.org/10.48550/arXiv.1601.04607$$DView paper in arXiv https://doi.org/10.1038/ncomms10295$$DView published paper (Access to full text may be restricted) |
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Snippet | Apart from being so far the only known binary multiferroic compound, CuO has a much higher transition temperature into the multiferroic state, 230 K, than any... Nat. Commun. 7, 10295 (2016) Apart from being so far the only known binary multiferroic compound, CuO has a much higher transition temperature into the... |
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SubjectTerms | Crosstalk Electric polarization Ferroelectric materials Ferroelectricity Magnetic fields Multiferroic materials Phase transitions Physics - Materials Science Transition temperature |
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Title | Magnetoelectric effect and phase transitions in CuO in external magnetic fields |
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