Radiation impact assessment of naturally occurring radionuclides and magnetic mineral studies of Bharathapuzha river sediments, South India

• Published in: Environmental earth sciences Vol. 71; no. 8; pp. 3593 - 3604
• Main Authors: Krishnamoorthy, N, Mullainathan, S, Mehra, R, Chaparro, Marcos A. E, Chaparro, Mauro A. E
• Format: Journal Article
• Language: English
• Published: Berlin/Heidelberg Springer-Verlag 01.04.2014; Springer Berlin Heidelberg; Springer; Springer Nature B.V
• Subjects: Biogeosciences; Bottom sediments; construction materials; Earth and Environmental Science; Earth Sciences; Earth, ocean, space; Engineering and environment geology. Geothermics; Environmental Science and Engineering; Exact sciences and technology; Fluvial sediments; Freshwater; Geochemistry; Geology; Hydrology/Water Resources; Isotope geochemistry; Isotope geochemistry. Geochronology; Magnetic fields; Marine and continental quaternary; Minerals; Original Article; Pollution, environment geology; Radiation; Radiation hazards; Radioactivity; radionuclides; Radium; Rivers; Sediment samplers; Sediments; Spectrometry; Statistical analysis; Surficial geology; Terrestrial Pollution; Water analysis; India; Asia; India, Kerala, Bharathapuzha; Hazard indices; Bharathapuzha river; River sediments; Fuzzy c-means clustering; Natural radioactivity; Magnetic susceptibility; rivers; stream transport; Ra-226; magnetic minerals; radium; concentration; air; radionucleids; alluvium; magnetic susceptibility; statistical analysis; K-40; Th-232; high resolution; radioactivity
• ISSN: 1866-6280; 1866-6299
• DOI: 10.1007/s12665-013-2751-y

The natural radioactivity levels and magnetic measurements in sediment samples of Bharathapuzha river for the first time have been determined. Bottom sediments from 33 locations were collected to determine ²²⁶Ra, ²³²Th and ⁴⁰K using a HPGe detector based on the high-resolution gamma spectrometry system, and magnetic susceptibility by using Bartington MS2 magnetic susceptibility meter. The calculated activity concentrations of ²²⁶Ra, ²³²Th and ⁴⁰K have been found to vary from 21.21 to 66.03 Bq kg⁻¹, 33.49 to 93.10 Bq kg⁻¹ and 232.25 to 899.66 Bq kg⁻¹, respectively. The results have been compared with worldwide recommended values and also with radioactivity measurements in river sediments of India and other parts of the world. The air-absorbed dose rate, indoor and outdoor annual effective dose rates and radium equivalent activity are calculated with an aim to access the radiation hazards arising due to the use of these materials in the construction of buildings and their mean values obtained are 74.83 nGy h⁻¹, 367.08 μSv y⁻¹, 91.77 μSv y⁻¹ and 157.09 Bq kg⁻¹, respectively. The mass-specific magnetic susceptibility values ranged widely from 35.4 to 2,160.5 × 10⁻⁸ m³ kg⁻¹ and compared with other rivers in South India. Multivariate statistical analyses were performed to describe the magnetic and radioactivity relevance of the different groups of samples. The data obtained in the present study may be useful for radiological and magnetic mapping of the study area in the future.