Photoluminescent Anisotropy Amplification in Polymorphic Organic Nanocrystals by Light-Harvesting Energy Transfer
Polymorphism and anisotropy are fundamental phenomena of crystalline materials. However, the structure-dependent photoluminescent (PL) anisotropy in polymorphic organic crystals has remained unexplored. Herein, two polymorphic nanocrystals, green-emitting nanorods (PtD-g) and yellow-emitting nanopla...
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| Published in | Journal of the American Chemical Society Vol. 141; no. 15; pp. 6157 - 6161 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
WASHINGTON
American Chemical Society
17.04.2019
Amer Chemical Soc |
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| Online Access | Get full text |
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| Abstract | Polymorphism and anisotropy are fundamental phenomena of crystalline materials. However, the structure-dependent photoluminescent (PL) anisotropy in polymorphic organic crystals has remained unexplored. Herein, two polymorphic nanocrystals, green-emitting nanorods (PtD-g) and yellow-emitting nanoplates (PtD-y), were obtained from a platinum(II)−β-diketonate complex. The PtD-y crystals display remarkable PL anisotropy with an anisotropy ratio of up to 0.87 whereas the emission of the PtD-g crystals is nearly unpolarized. The polarization properties are rationalized on the different molecular packing of these crystals. By light-harvesting energy transfer, the PtD-y crystals are successfully used to amplify the emission polarization of a red-emitting platinum acceptor (PtA) doped into the donor crystalline matrix, which is otherwise weakly polarized as pure crystals. |
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| AbstractList | Polymorphism and anisotropy are fundamental phenomena of crystalline materials. However, the structure-dependent photoluminescent (PL) anisotropy in polymorphic organic crystals has remained unexplored. Herein, two polymorphic nanocrystals, green-emitting nanorods (PtD-g) and yellow-emitting nanoplates (PtD-y), were obtained from a platinum(II)−β-diketonate complex. The PtD-y crystals display remarkable PL anisotropy with an anisotropy ratio of up to 0.87 whereas the emission of the PtD-g crystals is nearly unpolarized. The polarization properties are rationalized on the different molecular packing of these crystals. By light-harvesting energy transfer, the PtD-y crystals are successfully used to amplify the emission polarization of a red-emitting platinum acceptor (PtA) doped into the donor crystalline matrix, which is otherwise weakly polarized as pure crystals. Polymorphism and anisotropy are fundamental phenomena of crystalline materials. However, the structure-dependent photoluminescent (PL) anisotropy in polymorphic organic crystals has remained unexplored. Herein, two polymorphic nanocrystals, green-emitting nanorods (PtD-g) and yellow-emitting nanoplates (PtD-y), were obtained from a platinum(II)−β-diketonate complex. The PtD-y crystals display remarkable PL anisotropy with an anisotropy ratio of up to 0.87 whereas the emission of the PtD-g crystals is nearly unpolarized. The polarization properties are rationalized on the different molecular packing of these crystals. By light-harvesting energy transfer, the PtD-y crystals are successfully used to amplify the emission polarization of a red-emitting platinum acceptor (PtA) doped into the donor crystalline matrix, which is otherwise weakly polarized as pure crystals. Polymorphism and anisotropy are fundamental phenomena of crystalline materials. However, the structure-dependent photoluminescent (PL) anisotropy in polymorphic organic crystals has remained unexplored. Herein, two polymorphic nanocrystals, green-emitting nanorods (PtD-g) and yellow-emitting nanoplates (PtD-y), were obtained from a platinum(II)-β-diketonate complex. The PtD-y crystals display remarkable PL anisotropy with an anisotropy ratio of up to 0.87 whereas the emission of the PtD-g crystals is nearly unpolarized. The polarization properties are rationalized on the different molecular packing of these crystals. By light-harvesting energy transfer, the PtD-y crystals are successfully used to amplify the emission polarization of a red-emitting platinum acceptor (PtA) doped into the donor crystalline matrix, which is otherwise weakly polarized as pure crystals.Polymorphism and anisotropy are fundamental phenomena of crystalline materials. However, the structure-dependent photoluminescent (PL) anisotropy in polymorphic organic crystals has remained unexplored. Herein, two polymorphic nanocrystals, green-emitting nanorods (PtD-g) and yellow-emitting nanoplates (PtD-y), were obtained from a platinum(II)-β-diketonate complex. The PtD-y crystals display remarkable PL anisotropy with an anisotropy ratio of up to 0.87 whereas the emission of the PtD-g crystals is nearly unpolarized. The polarization properties are rationalized on the different molecular packing of these crystals. By light-harvesting energy transfer, the PtD-y crystals are successfully used to amplify the emission polarization of a red-emitting platinum acceptor (PtA) doped into the donor crystalline matrix, which is otherwise weakly polarized as pure crystals. Polymorphism and anisotropy are fundamental phenomena of crystalline materials. However, the structure-dependent photoluminescent (PL) anisotropy in polymorphic organic crystals has remained unexplored. Herein, two polymorphic nanocrystals, green-emitting nanorods (PtD-g) and yellow-emitting nanoplates (PtD-y), were obtained from a platinum(II)-beta-diketonate complex. The PtD-y crystals display remarkable PL anisotropy with an anisotropy ratio of up to 0.87 whereas the emission of the PtD-g crystals is nearly unpolarized. The polarization properties are rationalized on the different molecular packing of these crystals. By light-harvesting energy transfer, the PtD-y crystals are successfully used to amplify the emission polarization of a red-emitting platinum acceptor (PtA) doped into the donor crystalline matrix, which is otherwise weakly polarized as pure crystals. Polymorphism and anisotropy are fundamental phenomena of crystalline materials. However, the structure-dependent photoluminescent (PL) anisotropy in polymorphic organic crystals has remained unexplored. Herein, two polymorphic nanocrystals, green-emitting nanorods (PtD-g) and yellow-emitting nanoplates (PtD-y), were obtained from a platinum(II)-β-diketonate complex. The PtD-y crystals display remarkable PL anisotropy with an anisotropy ratio of up to 0.87 whereas the emission of the PtD-g crystals is nearly unpolarized. The polarization properties are rationalized on the different molecular packing of these crystals. By light-harvesting energy transfer, the PtD-y crystals are successfully used to amplify the emission polarization of a red-emitting platinum acceptor (PtA) doped into the donor crystalline matrix, which is otherwise weakly polarized as pure crystals. |
| Author | Zhao, Yong Sheng Zeng, Wei Liu, Yingying Sun, Meng-Jia Zhong, Yu-Wu Yao, Jiannian |
| AuthorAffiliation | Key Laboratory of Photochemistry, Beijing National Laboratory for Molecular Sciences, CAS Research/Education Center for Excellence in Molecular Sciences University of Chinese Academy of Sciences |
| AuthorAffiliation_xml | – name: University of Chinese Academy of Sciences – name: Key Laboratory of Photochemistry, Beijing National Laboratory for Molecular Sciences, CAS Research/Education Center for Excellence in Molecular Sciences |
| Author_xml | – sequence: 1 givenname: Meng-Jia surname: Sun fullname: Sun, Meng-Jia organization: University of Chinese Academy of Sciences – sequence: 2 givenname: Yingying surname: Liu fullname: Liu, Yingying organization: University of Chinese Academy of Sciences – sequence: 3 givenname: Wei surname: Zeng fullname: Zeng, Wei organization: University of Chinese Academy of Sciences – sequence: 4 givenname: Yong Sheng orcidid: 0000-0002-4329-0103 surname: Zhao fullname: Zhao, Yong Sheng email: zhongyuwu@iccas.ac.cn organization: University of Chinese Academy of Sciences – sequence: 5 givenname: Yu-Wu orcidid: 0000-0003-0712-0374 surname: Zhong fullname: Zhong, Yu-Wu email: yszhao@iccas.ac.cn organization: University of Chinese Academy of Sciences – sequence: 6 givenname: Jiannian surname: Yao fullname: Yao, Jiannian email: jnyao@iccas.ac.cn organization: University of Chinese Academy of Sciences |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/30945852$$D View this record in MEDLINE/PubMed |
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| SubjectTerms | anisotropy Chemistry Chemistry, Multidisciplinary energy transfer nanocrystals nanorods photoluminescence Physical Sciences platinum Science & Technology |
| Title | Photoluminescent Anisotropy Amplification in Polymorphic Organic Nanocrystals by Light-Harvesting Energy Transfer |
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