Ortho- and Para-Selective Ruthenium-Catalyzed C(sp2)–H Oxygenations of Phenol Derivatives
Versatile ruthenium catalysts allowed for efficient direct oxygenations of aryl carbamates under remarkably mild reaction conditions. In addition to chelation-assisted C–H activation, the optimized ruthenium catalyst proved amenable to para-selective hydroxylations of anisoles without Lewis basic di...
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| Published in | Organic letters Vol. 15; no. 13; pp. 3484 - 3486 |
|---|---|
| Main Authors | , |
| Format | Journal Article |
| Language | English |
| Published |
WASHINGTON
American Chemical Society
05.07.2013
Amer Chemical Soc |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Versatile ruthenium catalysts allowed for efficient direct oxygenations of aryl carbamates under remarkably mild reaction conditions. In addition to chelation-assisted C–H activation, the optimized ruthenium catalyst proved amenable to para-selective hydroxylations of anisoles without Lewis basic directing groups. |
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| AbstractList | Versatile ruthenium catalysts allowed for efficient direct oxygenations of aryl carbamates under remarkably mild reaction conditions. In addition to chelation-assisted C-H activation, the optimized ruthenium catalyst proved amenable to para-selective hydroxylations of anisoles without Lewis basic directing groups.Versatile ruthenium catalysts allowed for efficient direct oxygenations of aryl carbamates under remarkably mild reaction conditions. In addition to chelation-assisted C-H activation, the optimized ruthenium catalyst proved amenable to para-selective hydroxylations of anisoles without Lewis basic directing groups. Versatile ruthenium catalysts allowed for efficient direct oxygenations of aryl carbamates under remarkably mild reaction conditions. In addition to chelation-assisted C-H activation, the optimized ruthenium catalyst proved amenable to para-selective hydroxylations of anisoles without Lewis basic directing groups. |
| Author | Liu, Weiping Ackermann, Lutz |
| AuthorAffiliation | Georg-August-Universität |
| AuthorAffiliation_xml | – name: Georg-August-Universität |
| Author_xml | – sequence: 1 givenname: Weiping surname: Liu fullname: Liu, Weiping – sequence: 2 givenname: Lutz surname: Ackermann fullname: Ackermann, Lutz email: Lutz.Ackermann@chemie.uni-goettingen.de |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/23799802$$D View this record in MEDLINE/PubMed |
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| Keywords | H BOND ACTIVATION HYDROXYLATED ARENES FUNCTIONALIZATION CLEAVAGES PALLADIUM CONSTRUCTION ALKOXYLATION DIRECT ARYLATIONS CONTAINING HETEROCYCLES C-H |
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| Snippet | Versatile ruthenium catalysts allowed for efficient direct oxygenations of aryl carbamates under remarkably mild reaction conditions. In addition to... |
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| SubjectTerms | carbamates carbon-hydrogen bond activation catalysts chemical reactions chemical structure Chemistry Chemistry, Organic phenol Physical Sciences ruthenium Science & Technology |
| Title | Ortho- and Para-Selective Ruthenium-Catalyzed C(sp2)–H Oxygenations of Phenol Derivatives |
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