Quasi-Periodic Nanoripples in Graphene Grown by Chemical Vapor Deposition and Its Impact on Charge Transport
The technical breakthrough in synthesizing graphene by chemical vapor deposition methods (CVD) has opened up enormous opportunities for large-scale device applications. To improve the electrical properties of CVD graphene grown on copper (Cu-CVD graphene), recent efforts have focused on increasing t...
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Published in | ACS nano Vol. 6; no. 2; pp. 1158 - 1164 |
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Main Authors | , , , , , , , , , , |
Format | Journal Article |
Language | English |
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American Chemical Society
28.02.2012
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Abstract | The technical breakthrough in synthesizing graphene by chemical vapor deposition methods (CVD) has opened up enormous opportunities for large-scale device applications. To improve the electrical properties of CVD graphene grown on copper (Cu-CVD graphene), recent efforts have focused on increasing the grain size of such polycrystalline graphene films to 100 μm and larger. While an increase in grain size and, hence, a decrease of grain boundary density is expected to greatly enhance the device performance, here we show that the charge mobility and sheet resistance of Cu-CVD graphene is already limited within a single grain. We find that the current high-temperature growth and wet transfer methods of CVD graphene result in quasi-periodic nanoripple arrays (NRAs). Electron-flexural phonon scattering in such partially suspended graphene devices introduces anisotropic charge transport and sets limits to both the highest possible charge mobility and lowest possible sheet resistance values. Our findings provide guidance for further improving the CVD graphene growth and transfer process. |
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AbstractList | The technical breakthrough in synthesizing graphene by chemical vapor deposition methods (CVD) has opened up enormous opportunities for large-scale device applications. To improve the electrical properties of CVD graphene grown on copper (Cu-CVD graphene), recent efforts have focused on increasing the grain size of such polycrystalline graphene films to 100 μm and larger. While an increase in grain size and, hence, a decrease of grain boundary density is expected to greatly enhance the device performance, here we show that the charge mobility and sheet resistance of Cu-CVD graphene is already limited within a single grain. We find that the current high-temperature growth and wet transfer methods of CVD graphene result in quasi-periodic nanoripple arrays (NRAs). Electron-flexural phonon scattering in such partially suspended graphene devices introduces anisotropic charge transport and sets limits to both the highest possible charge mobility and lowest possible sheet resistance values. Our findings provide guidance for further improving the CVD graphene growth and transfer process. The technical breakthrough in synthesizing graphene by chemical vapor deposition methods (CVD) has opened up enormous opportunities for large-scale device applications. To improve the electrical properties of CVD graphene grown on copper (Cu-CVD graphene), recent efforts have focused on increasing the grain size of such polycrystalline graphene films to 100 mu m and larger. While an increase in grain size and, hence, a decrease of grain boundary density is expected to greatly enhance the device performance, here we show that the charge mobility and sheet resistance of Cu-CVD graphene is already limited within a single grain. We find that the current high-temperature growth and wet transfer methods of CVD graphene result in quasi-periodic nanoripple arrays (NRAs). Electron-flexural phonon scattering in such partially suspended graphene devices introduces anisotropic charge transport and sets limits to both the highest possible charge mobility and lowest possible sheet resistance values. Our findings provide guidance for further improving the CVD graphene growth and transfer process. |
Author | Ni, Guang-Xin Bae, Sukang Pachoud, Alexandre Kim, Hye Ri Hong, Byung Hee Kim, Young Soo Zheng, Yi Tan, Chang-Ling Ahn, Jong-Hyun Özyilmaz, Barbaros Im, Danho |
AuthorAffiliation | Department of Chemistry National University of Singapore School of Advanced Materials Science and Engineering SKKU Advanced Institute of Nanotechnology (SAINT) and Center for Human Interface Nano Technology (HINT) Sungkyunkwan University Seoul National University Department of Physics |
AuthorAffiliation_xml | – name: School of Advanced Materials Science and Engineering – name: – name: Sungkyunkwan University – name: Department of Chemistry – name: SKKU Advanced Institute of Nanotechnology (SAINT) and Center for Human Interface Nano Technology (HINT) – name: Department of Physics – name: National University of Singapore – name: Seoul National University |
Author_xml | – sequence: 1 givenname: Guang-Xin surname: Ni fullname: Ni, Guang-Xin – sequence: 2 givenname: Yi surname: Zheng fullname: Zheng, Yi – sequence: 3 givenname: Sukang surname: Bae fullname: Bae, Sukang – sequence: 4 givenname: Hye Ri surname: Kim fullname: Kim, Hye Ri – sequence: 5 givenname: Alexandre surname: Pachoud fullname: Pachoud, Alexandre – sequence: 6 givenname: Young Soo surname: Kim fullname: Kim, Young Soo – sequence: 7 givenname: Chang-Ling surname: Tan fullname: Tan, Chang-Ling – sequence: 8 givenname: Danho surname: Im fullname: Im, Danho – sequence: 9 givenname: Jong-Hyun surname: Ahn fullname: Ahn, Jong-Hyun – sequence: 10 givenname: Byung Hee surname: Hong fullname: Hong, Byung Hee email: barbaros@nus.edu.sg, byunghee@snu.ac.kr – sequence: 11 givenname: Barbaros surname: Özyilmaz fullname: Özyilmaz, Barbaros email: barbaros@nus.edu.sg, byunghee@snu.ac.kr |
BackLink | https://www.ncbi.nlm.nih.gov/pubmed/22251076$$D View this record in MEDLINE/PubMed |
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Keywords | flexural phonon scattering sheet resistance quasi-periodic nanoripple arrays transparent electrodes anisotropic charge transport CVD graphene |
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Snippet | The technical breakthrough in synthesizing graphene by chemical vapor deposition methods (CVD) has opened up enormous opportunities for large-scale device... |
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SubjectTerms | Charge Charge transport Chemical vapor deposition Copper Devices Electrical resistivity Grain size Graphene Nanostructure |
Title | Quasi-Periodic Nanoripples in Graphene Grown by Chemical Vapor Deposition and Its Impact on Charge Transport |
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