Photoluminescence Imaging of Suspended Single-Walled Carbon Nanotubes
Single-walled carbon nanotubes (SWNTs) suspended in air over trenches are imaged using their intrinsic near-infrared (NIR) photoluminescence (1.0−1.6 μm). Far-field emission from extended suspended lengths (∼50 μm) is both spatially and spectrally resolved, and SWNTs are classified based on the spat...
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| Published in | Nano letters Vol. 6; no. 8; pp. 1603 - 1608 |
|---|---|
| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
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Washington, DC
American Chemical Society
01.08.2006
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| Abstract | Single-walled carbon nanotubes (SWNTs) suspended in air over trenches are imaged using their intrinsic near-infrared (NIR) photoluminescence (1.0−1.6 μm). Far-field emission from extended suspended lengths (∼50 μm) is both spatially and spectrally resolved, and SWNTs are classified based on the spatial uniformity of their emission intensity and emission wavelength. In a few cases, emission assigned to different (n,m) species is observed along the same suspended segment. Most SWNTs imaged on millisecond time scales show steady emission, but a few fluctuate and suffer a reduction of intensity. The quantum efficiency is dramatically higher than that in previous reports and is estimated at 7%, a value that is precise but subject to corrections because of assumptions about absorption and coherence. |
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| AbstractList | Single-walled carbon nanotubes (SWNTs) suspended in air over trenches are imaged using their intrinsic near-infrared (NIR) photoluminescence (1.0-1.6 microm). Far-field emission from extended suspended lengths (approximately 50 microm) is both spatially and spectrally resolved, and SWNTs are classified based on the spatial uniformity of their emission intensity and emission wavelength. In a few cases, emission assigned to different (n,m) species is observed along the same suspended segment. Most SWNTs imaged on millisecond time scales show steady emission, but a few fluctuate and suffer a reduction of intensity. The quantum efficiency is dramatically higher than that in previous reports and is estimated at 7%, a value that is precise but subject to corrections because of assumptions about absorption and coherence.Single-walled carbon nanotubes (SWNTs) suspended in air over trenches are imaged using their intrinsic near-infrared (NIR) photoluminescence (1.0-1.6 microm). Far-field emission from extended suspended lengths (approximately 50 microm) is both spatially and spectrally resolved, and SWNTs are classified based on the spatial uniformity of their emission intensity and emission wavelength. In a few cases, emission assigned to different (n,m) species is observed along the same suspended segment. Most SWNTs imaged on millisecond time scales show steady emission, but a few fluctuate and suffer a reduction of intensity. The quantum efficiency is dramatically higher than that in previous reports and is estimated at 7%, a value that is precise but subject to corrections because of assumptions about absorption and coherence. Single-walled carbon nanotubes (SWNTs) suspended in air over trenches are imaged using their intrinsic near-infrared (NIR) photoluminescence (1.0-1.6 microm). Far-field emission from extended suspended lengths (approximately 50 microm) is both spatially and spectrally resolved, and SWNTs are classified based on the spatial uniformity of their emission intensity and emission wavelength. In a few cases, emission assigned to different (n,m) species is observed along the same suspended segment. Most SWNTs imaged on millisecond time scales show steady emission, but a few fluctuate and suffer a reduction of intensity. The quantum efficiency is dramatically higher than that in previous reports and is estimated at 7%, a value that is precise but subject to corrections because of assumptions about absorption and coherence. Single-walled carbon nanotubes (SWNTs) suspended in air over trenches are imaged using their intrinsic near-infrared (NIR) photoluminescence (1.0−1.6 μm). Far-field emission from extended suspended lengths (∼50 μm) is both spatially and spectrally resolved, and SWNTs are classified based on the spatial uniformity of their emission intensity and emission wavelength. In a few cases, emission assigned to different (n,m) species is observed along the same suspended segment. Most SWNTs imaged on millisecond time scales show steady emission, but a few fluctuate and suffer a reduction of intensity. The quantum efficiency is dramatically higher than that in previous reports and is estimated at 7%, a value that is precise but subject to corrections because of assumptions about absorption and coherence. |
| Author | Lefebvre, Jacques Austing, David G Bond, Jeffery Finnie, Paul |
| Author_xml | – sequence: 1 givenname: Jacques surname: Lefebvre fullname: Lefebvre, Jacques – sequence: 2 givenname: David G surname: Austing fullname: Austing, David G – sequence: 3 givenname: Jeffery surname: Bond fullname: Bond, Jeffery – sequence: 4 givenname: Paul surname: Finnie fullname: Finnie, Paul |
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| Copyright | Copyright © 2006 American Chemical Society 2007 INIST-CNRS |
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| Keywords | Near infrared radiation Singlewalled nanotube Near infrared spectrum Photoluminescence Far field Field emission Infrared spectra Quantum yield Spatial resolution |
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| Snippet | Single-walled carbon nanotubes (SWNTs) suspended in air over trenches are imaged using their intrinsic near-infrared (NIR) photoluminescence (1.0−1.6 μm).... Single-walled carbon nanotubes (SWNTs) suspended in air over trenches are imaged using their intrinsic near-infrared (NIR) photoluminescence (1.0-1.6 microm).... |
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| SubjectTerms | Condensed matter: electronic structure, electrical, magnetic, and optical properties Cross-disciplinary physics: materials science; rheology Electron and ion emission by liquids and solids; impact phenomena Exact sciences and technology Field emission, ionization, evaporation, and desorption Light Luminescent Measurements - methods Materials science Materials Testing - methods Microscopy, Fluorescence - methods Nanoscale materials and structures: fabrication and characterization Nanotechnology - methods Nanotubes Nanotubes, Carbon - analysis Nanotubes, Carbon - chemistry Nanotubes, Carbon - radiation effects Nanotubes, Carbon - ultrastructure Optical properties and condensed-matter spectroscopy and other interactions of matter with particles and radiation Photoluminescence Physics Spectrometry, Fluorescence - methods |
| Title | Photoluminescence Imaging of Suspended Single-Walled Carbon Nanotubes |
| URI | http://dx.doi.org/10.1021/nl060530e https://www.ncbi.nlm.nih.gov/pubmed/16895343 https://www.proquest.com/docview/68720992 |
| Volume | 6 |
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