Photoconductivity Multiplication in Semiconducting Few-Layer MoTe2

We report efficient photoconductivity multiplication in few-layer 2H-MoTe2 as a direct consequence of an efficient steplike carrier multiplication with near unity quantum yield and high carrier mobility (∼45 cm2 V–1 s–1) in MoTe2. This photoconductivity multiplication is quantified using ultrafast,...

Full description

Saved in:
Bibliographic Details
Published inNano letters Vol. 20; no. 8; pp. 5807 - 5813
Main Authors Zheng, Wenhao, Bonn, Mischa, Wang, Hai I
Format Journal Article
LanguageEnglish
Published American Chemical Society 12.08.2020
Subjects
Online AccessGet full text

Cover

Loading…
Abstract We report efficient photoconductivity multiplication in few-layer 2H-MoTe2 as a direct consequence of an efficient steplike carrier multiplication with near unity quantum yield and high carrier mobility (∼45 cm2 V–1 s–1) in MoTe2. This photoconductivity multiplication is quantified using ultrafast, excitation-wavelength-dependent photoconductivity measurements employing contact-free terahertz spectroscopy. We discuss the possible origins of efficient carrier multiplication in MoTe2 to guide future theoretical investigations. The combination of photoconductivity multiplication and the advantageous bandgap renders MoTe2 as a promising candidate for efficient optoelectronic devices.
AbstractList We report efficient photoconductivity multiplication in few-layer 2H-MoTe2 as a direct consequence of an efficient steplike carrier multiplication with near unity quantum yield and high carrier mobility (∼45 cm2 V–1 s–1) in MoTe2. This photoconductivity multiplication is quantified using ultrafast, excitation-wavelength-dependent photoconductivity measurements employing contact-free terahertz spectroscopy. We discuss the possible origins of efficient carrier multiplication in MoTe2 to guide future theoretical investigations. The combination of photoconductivity multiplication and the advantageous bandgap renders MoTe2 as a promising candidate for efficient optoelectronic devices.
We report efficient photoconductivity multiplication in few-layer 2H-MoTe 2 as a direct consequence of an efficient steplike carrier multiplication with near unity quantum yield and high carrier mobility (∼45 cm 2 V –1 s –1 ) in MoTe 2 . This photoconductivity multiplication is quantified using ultrafast, excitation-wavelength-dependent photoconductivity measurements employing contact-free terahertz spectroscopy. We discuss the possible origins of efficient carrier multiplication in MoTe 2 to guide future theoretical investigations. The combination of photoconductivity multiplication and the advantageous bandgap renders MoTe 2 as a promising candidate for efficient optoelectronic devices.
We report efficient photoconductivity multiplication in few-layer 2H-MoTe2 as a direct consequence of an efficient steplike carrier multiplication with near unity quantum yield and high carrier mobility (∼45 cm2 V-1 s-1) in MoTe2. This photoconductivity multiplication is quantified using ultrafast, excitation-wavelength-dependent photoconductivity measurements employing contact-free terahertz spectroscopy. We discuss the possible origins of efficient carrier multiplication in MoTe2 to guide future theoretical investigations. The combination of photoconductivity multiplication and the advantageous bandgap renders MoTe2 as a promising candidate for efficient optoelectronic devices.We report efficient photoconductivity multiplication in few-layer 2H-MoTe2 as a direct consequence of an efficient steplike carrier multiplication with near unity quantum yield and high carrier mobility (∼45 cm2 V-1 s-1) in MoTe2. This photoconductivity multiplication is quantified using ultrafast, excitation-wavelength-dependent photoconductivity measurements employing contact-free terahertz spectroscopy. We discuss the possible origins of efficient carrier multiplication in MoTe2 to guide future theoretical investigations. The combination of photoconductivity multiplication and the advantageous bandgap renders MoTe2 as a promising candidate for efficient optoelectronic devices.
Author Bonn, Mischa
Wang, Hai I
Zheng, Wenhao
Author_xml – sequence: 1
  givenname: Wenhao
  surname: Zheng
  fullname: Zheng, Wenhao
– sequence: 2
  givenname: Mischa
  orcidid: 0000-0001-6851-8453
  surname: Bonn
  fullname: Bonn, Mischa
– sequence: 3
  givenname: Hai I
  orcidid: 0000-0003-0940-3984
  surname: Wang
  fullname: Wang, Hai I
  email: wanghai@mpip-mainz.mpg.de
BookMark eNpVkF1LwzAUhoNM3If-Ay966U1nvrPcCDqcChsKzuuQpumW0SazTSf793ZsE7w6h_M-vHCeIej54C0AtwiOEcToXptm7LUPpY1xDA1EXJILMECMwJRLiXt_-4T2wbBpNhBCSRi8An2CuRQIogF4-liHGEzweWui27m4TxZtGd22dEZHF3zifPJpK3dG_CqZ2Z90rve2ThZhafE1uCx02dib0xyBr9nzcvqazt9f3qaP81QTyWPKLGXCZFpzxmRudYYog6LAPOMZMcZInheC6YIgmWFDWD4ReY4I1ijDHBeMjMDDsXfbZpXNjfWx1qXa1q7S9V4F7dT_xLu1WoWdEpRNqBBdwd2poA7frW2iqlxjbFlqb0PbKEwxR4JJSjsUHtHOstqEtvbdZwpBdVCvDsezenVST34BsA59EQ
ContentType Journal Article
Copyright Copyright © 2020 American Chemical Society 2020 American Chemical Society
Copyright_xml – notice: Copyright © 2020 American Chemical Society 2020 American Chemical Society
DBID 7X8
5PM
DOI 10.1021/acs.nanolett.0c01693
DatabaseName MEDLINE - Academic
PubMed Central (Full Participant titles)
DatabaseTitle MEDLINE - Academic
DatabaseTitleList

MEDLINE - Academic
DeliveryMethod fulltext_linktorsrc
Discipline Engineering
EISSN 1530-6992
EndPage 5813
ExternalDocumentID PMC7458477
b424465026
GroupedDBID -
.K2
123
55A
5VS
7~N
AABXI
ABMVS
ABPTK
ABUCX
ACGFS
ACS
AEESW
AENEX
AFEFF
ALMA_UNASSIGNED_HOLDINGS
AQSVZ
BAANH
CS3
DU5
EBS
ED
ED~
F5P
GNL
IH9
IHE
JG
JG~
K2
PK8
RNS
ROL
TN5
UI2
VF5
VG9
W1F
X
---
-~X
4.4
6P2
7X8
AAHBH
ABBLG
ABJNI
ABLBI
ABQRX
ACBEA
ADHLV
AHGAQ
CUPRZ
GGK
5PM
ID FETCH-LOGICAL-a396t-5e457cbaa6559deab14507f26b6b3ccc96df75af319b2c35d87dd132a1b262f53
IEDL.DBID ACS
ISSN 1530-6984
1530-6992
IngestDate Thu Aug 21 14:07:43 EDT 2025
Fri Jul 11 01:38:12 EDT 2025
Thu Aug 27 13:41:55 EDT 2020
IsDoiOpenAccess true
IsOpenAccess true
IsPeerReviewed true
IsScholarly true
Issue 8
Keywords impact ionization
terahertz spectroscopy
carrier multiplication
transition metal dichalcogenides (TMDCs)
2D materials
MoTe2
Language English
License This is an open access article published under a Creative Commons Attribution (CC-BY) License, which permits unrestricted use, distribution and reproduction in any medium, provided the author and source are cited.
LinkModel DirectLink
MergedId FETCHMERGED-LOGICAL-a396t-5e457cbaa6559deab14507f26b6b3ccc96df75af319b2c35d87dd132a1b262f53
Notes ObjectType-Article-1
SourceType-Scholarly Journals-1
ObjectType-Feature-2
content type line 23
ORCID 0000-0001-6851-8453
0000-0003-0940-3984
OpenAccessLink https://pubmed.ncbi.nlm.nih.gov/PMC7458477
PMID 32697101
PQID 2426175944
PQPubID 23479
PageCount 7
ParticipantIDs pubmedcentral_primary_oai_pubmedcentral_nih_gov_7458477
proquest_miscellaneous_2426175944
acs_journals_10_1021_acs_nanolett_0c01693
ProviderPackageCode JG~
55A
AABXI
GNL
VF5
7~N
VG9
W1F
ACS
AEESW
AFEFF
.K2
ABMVS
ABUCX
IH9
BAANH
AQSVZ
ED~
UI2
PublicationCentury 2000
PublicationDate 2020-08-12
PublicationDateYYYYMMDD 2020-08-12
PublicationDate_xml – month: 08
  year: 2020
  text: 2020-08-12
  day: 12
PublicationDecade 2020
PublicationTitle Nano letters
PublicationTitleAlternate Nano Lett
PublicationYear 2020
Publisher American Chemical Society
Publisher_xml – name: American Chemical Society
SSID ssj0009350
Score 2.5458968
Snippet We report efficient photoconductivity multiplication in few-layer 2H-MoTe2 as a direct consequence of an efficient steplike carrier multiplication with near...
We report efficient photoconductivity multiplication in few-layer 2H-MoTe 2 as a direct consequence of an efficient steplike carrier multiplication with near...
SourceID pubmedcentral
proquest
acs
SourceType Open Access Repository
Aggregation Database
Publisher
StartPage 5807
SubjectTerms Letter
Title Photoconductivity Multiplication in Semiconducting Few-Layer MoTe2
URI http://dx.doi.org/10.1021/acs.nanolett.0c01693
https://www.proquest.com/docview/2426175944
https://pubmed.ncbi.nlm.nih.gov/PMC7458477
Volume 20
hasFullText 1
inHoldings 1
isFullTextHit
isPrint
link http://utb.summon.serialssolutions.com/2.0.0/link/0/eLvHCXMwlV1bS8MwFA46X_TBuzhvVPDFh9Q2zaV9nMMxxKmwDfZWkjR1Q0jFdgj-epO2Y6si6GtbQpOc0_N9PSffAeCKICI8hijEQRpBnHIPRgkmUJgvnyeZUH7ZkmXwSPtjfD8hkyVR_J7BR_4Nl7mruc7MNArXk6V6yDrYQDRklmx1usOlyG5QdmQ1TmwoURTixVG5X0axAUnmDWjZLIxciTS9HfC0OK9TFZi8uvNCuPLzp3zjHyexC7Zr0Ol0KivZA2tK74OtFSnCA3D7PM2KzJBjq_9aNpRwBlWtYf1Tz5lpZ2gr6etH9IvTUx_wgRvM7gyykUKHYNy7G3X7sO6vAHkQ0QIShQmTgnNqaEWiuPCxQYcpooKKQEoZ0SRlhKfGSwWSAUlCliSGvXJfIIpSEhyBls60OgaO70sSKc9TYWoYI8MhEonkJg4onhKWoDa4NksQ1_6Rx2XqG_mxvbhYl7helza4XGxIbGzdJjC4Vtk8jy2cMHAnwrgNWGOn4rdKmyO2atnNO3o2LVWzWZkRZif_eJNTsIksvbYKuOgMtIr3uTo3GKQQF6XhfQF7V9wd
linkProvider American Chemical Society
linkToHtml http://utb.summon.serialssolutions.com/2.0.0/link/0/eLvHCXMwzV1BT9swFH5C7LBx2AYM0Y2NIMFhh5TEsePmwKHrVhVo0SSKxM3YjrOiSc60pELb_9lf4Xfx7KZAkXbggMTViSzb7_n5e37P3wPYZYSpiJM0pEmRhbSQUZjllIUKLV-kuTKxL8kyOkkHZ_TonJ0vwb_5WxgcRIU9VT6If8cuEO-7NittibOp25H2JCJNLuWx-XOFnlp1cPgVxbpHSP_buDcIm2ICoUyytA6ZoYxrJWWKGDo3UsUUoVBBUpWqRGudpXnBmSxQJRXRCcs7PM_RVZOxIikpXHEItPQvEP8Q5-N1e6d33L6JLwSLtgM9saxD5y_0_jNqdw7qagHRLuZj3jvg-m_g-nZpfF7Lz_a0Vm399wFr5LNfu7fwuoHYQXe2J1Zhydg1WLlHvLgOX75PyrrUpXVst758RjCaZVY2V5jBpQ1O3buB5hf7I-ibq3Ao0UMJRuXYkHdw9iST2IBlW1qzCUEca5aZKDKdAv1jTjtE5VriqWdkwXhOWvAZl1w01qASPtBPYuEa53IQjRxasDPXA4E724VrpDXltBIOPCG4yyhtAV9QEPFrxkQiHDf44hd7OfEc4dzHv_n7R4xkG14OxqOhGB6eHH-AV8RdLDjuX7IFy_XvqfmI6KtWn7zuB3Dx1ApzAws_QBI
linkToPdf http://utb.summon.serialssolutions.com/2.0.0/link/0/eLvHCXMw1V1LT9wwEB4hKqH20AJtxZY-gkQPPWSbOHa8OfTAoytei5AAiZvrZ0GVHESyQvCP-lf4VYy92Zat1EMPHHp1Isv2jMffeMbfAKwzwlTGSZnSwlUpdTJLK0NZqtDyZZorm8eSLKPDcueU7p2xszn4OX0Lg4NosKcmBvHDrr40rmMYyD-Hdi99jTNq-5mORCJdPuW-vblGb635sruNov1IyPDrydZO2hUUSGVRlW3KLGVcKylLxNHGSpVThEOOlKpUhda6Ko3jTDpUS0V0wcyAG4PumswVKYkLBSLQ2j8JkcLg521sHf_m9y1iMVi0H-iNVQM6faX3l1GHs1A3M6h2NifzwSE3fAF3v5Yn5rb86I9b1de3fzBH_hfrtwjPO6idbEz2xhLMWb8Mzx4QML6EzaPzuq117QPrbSyjkYwmGZbdVWZy4ZPj8H6g-8V_T4b2Oj2Q6Kkko_rEkldw-iiTeA3zvvZ2BZI816yyWWYHDv1kTgdEGS3x9LPSMW5IDz7hkovOKjQiBvxJLkLjVA6ik0MP1qa6IHCHh7CN9LYeNyKAKAR5FaU94DNKIi4njCQicITPfvEX55ErnMc4OH_zDyP5AAtH20NxsHu4vwpPSbhfCBTA5C3Mt1dj-w5BWKveR_VP4Ntj68s9ePhClQ
openUrl ctx_ver=Z39.88-2004&ctx_enc=info%3Aofi%2Fenc%3AUTF-8&rfr_id=info%3Asid%2Fsummon.serialssolutions.com&rft_val_fmt=info%3Aofi%2Ffmt%3Akev%3Amtx%3Ajournal&rft.genre=article&rft.atitle=Photoconductivity+Multiplication+in+Semiconducting+Few-Layer+MoTe2&rft.jtitle=Nano+letters&rft.au=Zheng%2C+Wenhao&rft.au=Bonn%2C+Mischa&rft.au=Wang%2C+Hai+I.&rft.date=2020-08-12&rft.pub=American+Chemical+Society&rft.issn=1530-6984&rft.eissn=1530-6992&rft.volume=20&rft.issue=8&rft.spage=5807&rft.epage=5813&rft_id=info:doi/10.1021%2Facs.nanolett.0c01693&rft_id=info%3Apmid%2F32697101&rft.externalDocID=PMC7458477
thumbnail_l http://covers-cdn.summon.serialssolutions.com/index.aspx?isbn=/lc.gif&issn=1530-6984&client=summon
thumbnail_m http://covers-cdn.summon.serialssolutions.com/index.aspx?isbn=/mc.gif&issn=1530-6984&client=summon
thumbnail_s http://covers-cdn.summon.serialssolutions.com/index.aspx?isbn=/sc.gif&issn=1530-6984&client=summon