An Approach to Thermodynamically Controlled Supramolecular Assembly Possessing an Integral Locking Mechanism
A general approach for thermodynamically controlled molecular assembly employing carbonyl addition chemistry is exemplified with a prototypical rotaxane synthesis. Recognition−driven assembly of the rotaxane proceeds under conditions of mild base catalysis, while subsequent treatment with catalytic...
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| Published in | Journal of the American Chemical Society Vol. 131; no. 3; pp. 902 - 903 |
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| Main Authors | , |
| Format | Journal Article |
| Language | English |
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WASHINGTON
American Chemical Society
28.01.2009
Amer Chemical Soc |
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| Abstract | A general approach for thermodynamically controlled molecular assembly employing carbonyl addition chemistry is exemplified with a prototypical rotaxane synthesis. Recognition−driven assembly of the rotaxane proceeds under conditions of mild base catalysis, while subsequent treatment with catalytic acid triggers a dehydrative locking mechanism and fixes the evolved molecular architecture in place. |
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| AbstractList | A general approach for thermodynamically controlled molecular assembly employing carbonyl addition chemistry is exemplified with a prototypical rotaxane synthesis. Recognition-driven assembly of the rotaxane proceeds under conditions of mild base catalysis, while subsequent treatment with catalytic acid triggers a dehydrative locking mechanism and fixes the evolved molecular architecture in place. A general approach for thermodynamically controlled molecular assembly employing carbonyl addition chemistry is exemplified with a prototypical rotaxane synthesis. Recognition−driven assembly of the rotaxane proceeds under conditions of mild base catalysis, while subsequent treatment with catalytic acid triggers a dehydrative locking mechanism and fixes the evolved molecular architecture in place. |
| Author | Cagulada, Amy M Hamilton, Darren G |
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| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/19154171$$D View this record in MEDLINE/PubMed |
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| Title | An Approach to Thermodynamically Controlled Supramolecular Assembly Possessing an Integral Locking Mechanism |
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