CO2 Capture and Separations Using MOFs: Computational and Experimental Studies

This Review focuses on research oriented toward elucidation of the various aspects that determine adsorption of CO2 in metal–organic frameworks and its separation from gas mixtures found in industrial processes. It includes theoretical, experimental, and combined approaches able to characterize the...

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Published inChemical reviews Vol. 117; no. 14; pp. 9674 - 9754
Main Authors Yu, Jiamei, Xie, Lin-Hua, Li, Jian-Rong, Ma, Yuguang, Seminario, Jorge M, Balbuena, Perla B
Format Journal Article
LanguageEnglish
Published Easton American Chemical Society 26.07.2017
Subjects
Adsorbates
Adsorption
Carbon dioxide
Carbon sequestration
Chemical reactions
coordination polymers
Desorption
Experiments
Gas mixtures
Impurities
Membranes
Metal-organic frameworks
Stability analysis
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Summary:This Review focuses on research oriented toward elucidation of the various aspects that determine adsorption of CO2 in metal–organic frameworks and its separation from gas mixtures found in industrial processes. It includes theoretical, experimental, and combined approaches able to characterize the materials, investigate the adsorption/desorption/reaction properties of the adsorbates inside such environments, screen and design new materials, and analyze additional factors such as material regenerability, stability, effects of impurities, and cost among several factors that influence the effectiveness of the separations. CO2 adsorption, separations, and membranes are reviewed followed by an analysis of the effects of stability, impurities, and process operation conditions on practical applications.
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ISSN:0009-2665
1520-6890
1520-6890
DOI:10.1021/acs.chemrev.6b00626