Two Indium Iodate–Nitrates with Large Birefringence Induced by Hybrid Anionic Functional Groups and Their Favorable Arrangements
Two new indium iodate–nitrates, In(IO3)2(NO3) (1) and [In(IO3)(OH)(H2O)](NO3) (2), were rationally designed through the integration of hybrid anionic functional units. They exhibit large birefringences (1, 0.269; 2, 0.188, at 532 nm) and wide band gaps (1, 4.08 eV; 2, 4.39 eV), which is attribu...
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| Published in | Inorganic chemistry Vol. 61; no. 8; pp. 3374 - 3378 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
American Chemical Society
28.02.2022
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| Online Access | Get full text |
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| Abstract | Two new indium iodate–nitrates, In(IO3)2(NO3) (1) and [In(IO3)(OH)(H2O)](NO3) (2), were rationally designed through the integration of hybrid anionic functional units. They exhibit large birefringences (1, 0.269; 2, 0.188, at 532 nm) and wide band gaps (1, 4.08 eV; 2, 4.39 eV), which is attributed to the synergistic effect of two types of birefringence-active units, namely, lone-pair IO3 and π-conjugated NO3 anionic groups. Through the substitution of OH and H2O of 2 with IO3, the hydrogen bonds of 2 are eliminated and the birefringence of 1 is greatly enhanced, highlighting the intriguing role of isovalent substitution in the discovery of fascinating optical materials. |
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| AbstractList | Two new indium iodate-nitrates, In(IO
)
(NO
) (
) and [In(IO
)(OH)(H
O)](NO
) (
), were rationally designed through the integration of hybrid anionic functional units. They exhibit large birefringences (
, 0.269;
, 0.188, at 532 nm) and wide band gaps (
, 4.08 eV;
, 4.39 eV), which is attributed to the synergistic effect of two types of birefringence-active units, namely, lone-pair IO
and π-conjugated NO
anionic groups. Through the substitution of OH and H
O of
with IO
, the hydrogen bonds of
are eliminated and the birefringence of
is greatly enhanced, highlighting the intriguing role of isovalent substitution in the discovery of fascinating optical materials. Two new indium iodate–nitrates, In(IO3)2(NO3) (1) and [In(IO3)(OH)(H2O)](NO3) (2), were rationally designed through the integration of hybrid anionic functional units. They exhibit large birefringences (1, 0.269; 2, 0.188, at 532 nm) and wide band gaps (1, 4.08 eV; 2, 4.39 eV), which is attributed to the synergistic effect of two types of birefringence-active units, namely, lone-pair IO3 and π-conjugated NO3 anionic groups. Through the substitution of OH and H2O of 2 with IO3, the hydrogen bonds of 2 are eliminated and the birefringence of 1 is greatly enhanced, highlighting the intriguing role of isovalent substitution in the discovery of fascinating optical materials. Two new indium iodate-nitrates, In(IO3)2(NO3) (1) and [In(IO3)(OH)(H2O)](NO3) (2), were rationally designed through the integration of hybrid anionic functional units. They exhibit large birefringences (1, 0.269; 2, 0.188, at 532 nm) and wide band gaps (1, 4.08 eV; 2, 4.39 eV), which is attributed to the synergistic effect of two types of birefringence-active units, namely, lone-pair IO3 and π-conjugated NO3 anionic groups. Through the substitution of OH and H2O of 2 with IO3, the hydrogen bonds of 2 are eliminated and the birefringence of 1 is greatly enhanced, highlighting the intriguing role of isovalent substitution in the discovery of fascinating optical materials.Two new indium iodate-nitrates, In(IO3)2(NO3) (1) and [In(IO3)(OH)(H2O)](NO3) (2), were rationally designed through the integration of hybrid anionic functional units. They exhibit large birefringences (1, 0.269; 2, 0.188, at 532 nm) and wide band gaps (1, 4.08 eV; 2, 4.39 eV), which is attributed to the synergistic effect of two types of birefringence-active units, namely, lone-pair IO3 and π-conjugated NO3 anionic groups. Through the substitution of OH and H2O of 2 with IO3, the hydrogen bonds of 2 are eliminated and the birefringence of 1 is greatly enhanced, highlighting the intriguing role of isovalent substitution in the discovery of fascinating optical materials. |
| Author | Mao, Jiang-Gao Jiang, Ting-kun Hu, Chun-Li Huang, Yu Fang, Zhi Yang, Bing-Ping |
| AuthorAffiliation | College of Chemistry State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter University of Chinese Academy of Sciences |
| AuthorAffiliation_xml | – name: University of Chinese Academy of Sciences – name: College of Chemistry – name: State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter |
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| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/35156368$$D View this record in MEDLINE/PubMed |
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| Snippet | Two new indium iodate–nitrates, In(IO3)2(NO3) (1) and [In(IO3)(OH)(H2O)](NO3) (2), were rationally designed through the integration of hybrid anionic... Two new indium iodate-nitrates, In(IO ) (NO ) ( ) and [In(IO )(OH)(H O)](NO ) ( ), were rationally designed through the integration of hybrid anionic... Two new indium iodate-nitrates, In(IO3)2(NO3) (1) and [In(IO3)(OH)(H2O)](NO3) (2), were rationally designed through the integration of hybrid anionic... |
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| Title | Two Indium Iodate–Nitrates with Large Birefringence Induced by Hybrid Anionic Functional Groups and Their Favorable Arrangements |
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