Printable Light-Emitting Metasurfaces with Enhanced Directional Photoluminescence

• Published in: Nano letters Vol. 24; no. 19; pp. 5783 - 5790
• Main Authors: Jeong, Minsu, Ko, Byoungsu, Jung, Chunghwan, Kim, Jaekyung, Jang, Jaehyuck, Mun, Jungho, Lee, Jihae, Yun, Suhyeon, Kim, Sejeong, Rho, Junsuk
• Format: Journal Article
• Language: English
• Published: United States American Chemical Society 15.05.2024
• Subjects: quantum dot; particle-embedded resin; directional photoluminescence; nanoimprint lithography; resonant metasurface
• ISSN: 1530-6984; 1530-6992
• DOI: 10.1021/acs.nanolett.4c00871

Nanoimprint lithography is gaining popularity as a cost-efficient way to reproduce nanostructures in large quantities. Recent advances in nanoimprinting lithography using high-index nanoparticles have demonstrated replication of photonic devices, but it is difficult to confer special properties on nanostructures beyond general metasurfaces. Here, we introduce a novel method for fabricating light-emitting metasurfaces using nanoimprinting lithography. By utilizing quantum dots embedded in resin, we successfully imprint dielectric metasurfaces that function simultaneously as both emitters and resonators. This approach to incorporating quantum dots into metasurfaces demonstrates an improvement in photoluminescence characteristics compared to the situation where quantum dots and metasurfaces are independently incorporated. Design of the metasurface is specifically tailored to support photonic modes within the emission band of quantum dots with a large enhancement of photoluminescence. This study indicates that nanoimprinting lithography has the capability to construct nanostructures using functionalized nanoparticles and could be used in various fields of nanophotonic applications.